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Structural materials with afterglow room temperature phosphorescence activated by lignin oxidation

Author

Listed:
  • Keliang Wan

    (Northeast Forestry University, Ministry of Education)

  • Bing Tian

    (Northeast Forestry University, Ministry of Education)

  • Yingxiang Zhai

    (Northeast Forestry University, Ministry of Education)

  • Yuxuan Liu

    (Chinese Academy of Sciences)

  • He Wang

    (Nanjing Tech University)

  • Shouxin Liu

    (Northeast Forestry University, Ministry of Education)

  • Shujun Li

    (Northeast Forestry University, Ministry of Education)

  • Wenpeng Ye

    (Nanjing Tech University)

  • Zhongfu An

    (Nanjing Tech University)

  • Changzhi Li

    (Chinese Academy of Sciences)

  • Jian Li

    (Northeast Forestry University, Ministry of Education)

  • Tony D. James

    (University of Bath)

  • Zhijun Chen

    (Northeast Forestry University, Ministry of Education)

Abstract

Sustainable afterglow room temperature phosphorescence (RTP) materials, especially afterglow RTP structural materials, are crucial but remain difficult to achieve. Here, an oxidation strategy is developed to convert lignin to afterglow materials with a lifetime of ~ 408 ms. Specifically, lignin is oxidized to give aromatic chromophores and fatty acids using H2O2. The aromatic chromophores are locked by a fatty acid-based matrix by hydrogen bonds, triggering enhanced spin orbit coupling and long afterglow emission. More interestingly, motivated by this discovery, an auto fabrication line is built to convert wood (natural structural materials) to wood with afterglow RTP emission (RTP wood) via in situ oxidation of naturally-occurring lignin located in the wood cell walls to oxidized lignin (OL). The as-prepared RTP wood exhibits great potential for the construction of sustainable afterglow furniture. With this research we provide a new strategy to promote the sustainability of afterglow RTP materials and structural materials.

Suggested Citation

  • Keliang Wan & Bing Tian & Yingxiang Zhai & Yuxuan Liu & He Wang & Shouxin Liu & Shujun Li & Wenpeng Ye & Zhongfu An & Changzhi Li & Jian Li & Tony D. James & Zhijun Chen, 2022. "Structural materials with afterglow room temperature phosphorescence activated by lignin oxidation," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-33273-1
    DOI: 10.1038/s41467-022-33273-1
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    Cited by:

    1. Hongda Guo & Mengnan Cao & Ruixia Liu & Bing Tian & Shouxin Liu & Jian Li & Shujun Li & Bernd Strehmel & Tony D. James & Zhijun Chen, 2024. "Photocured room temperature phosphorescent materials from lignosulfonate," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    2. Tianhong Chen & Dongpeng Yan, 2024. "Full-color, time-valve controllable and Janus-type long-persistent luminescence from all-inorganic halide perovskites," Nature Communications, Nature, vol. 15(1), pages 1-13, December.

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