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Elastic conducting polymer composites in thermoelectric modules

Author

Listed:
  • Nara Kim

    (Linköping University)

  • Samuel Lienemann

    (Linköping University)

  • Ioannis Petsagkourakis

    (Linköping University)

  • Desalegn Alemu Mengistie

    (Linköping University
    California Polytechnic State University)

  • Seyoung Kee

    (The University of Auckland)

  • Thomas Ederth

    (Linköping University)

  • Viktor Gueskine

    (Linköping University)

  • Philippe Leclère

    (University of Mons)

  • Roberto Lazzaroni

    (University of Mons)

  • Xavier Crispin

    (Linköping University)

  • Klas Tybrandt

    (Linköping University)

Abstract

The rapid growth of wearables has created a demand for lightweight, elastic and conformal energy harvesting and storage devices. The conducting polymer poly(3,4-ethylenedioxythiophene) has shown great promise for thermoelectric generators, however, the thick layers of pristine poly(3,4-ethylenedioxythiophene) required for effective energy harvesting are too hard and brittle for seamless integration into wearables. Poly(3,4-ethylenedioxythiophene)-elastomer composites have been developed to improve its mechanical properties, although so far without simultaneously achieving softness, high electrical conductivity, and stretchability. Here we report an aqueously processed poly(3,4-ethylenedioxythiophene)-polyurethane-ionic liquid composite, which combines high conductivity (>140 S cm−1) with superior stretchability (>600%), elasticity, and low Young’s modulus (

Suggested Citation

  • Nara Kim & Samuel Lienemann & Ioannis Petsagkourakis & Desalegn Alemu Mengistie & Seyoung Kee & Thomas Ederth & Viktor Gueskine & Philippe Leclère & Roberto Lazzaroni & Xavier Crispin & Klas Tybrandt, 2020. "Elastic conducting polymer composites in thermoelectric modules," Nature Communications, Nature, vol. 11(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:11:y:2020:i:1:d:10.1038_s41467-020-15135-w
    DOI: 10.1038/s41467-020-15135-w
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    Cited by:

    1. Fan, Zeng & Zhang, Yaoyun & Pan, Lujun & Ouyang, Jianyong & Zhang, Qian, 2021. "Recent developments in flexible thermoelectrics: From materials to devices," Renewable and Sustainable Energy Reviews, Elsevier, vol. 137(C).
    2. Jiachen Wang & Yuto Ochiai & Niannian Wu & Kiyohiro Adachi & Daishi Inoue & Daisuke Hashizume & Desheng Kong & Naoji Matsuhisa & Tomoyuki Yokota & Qiang Wu & Wei Ma & Lulu Sun & Sixing Xiong & Baocai , 2024. "Intrinsically stretchable organic photovoltaics by redistributing strain to PEDOT:PSS with enhanced stretchability and interfacial adhesion," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    3. Yijie Liu & Xiaodong Wang & Shuaihang Hou & Zuoxu Wu & Jian Wang & Jun Mao & Qian Zhang & Zhiguo Liu & Feng Cao, 2023. "Scalable-produced 3D elastic thermoelectric network for body heat harvesting," Nature Communications, Nature, vol. 14(1), pages 1-8, December.

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