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Extremely stretchable and self-healing conductor based on thermoplastic elastomer for all-three-dimensional printed triboelectric nanogenerator

Author

Listed:
  • Kaushik Parida

    (Nanyang Technological University)

  • Gurunathan Thangavel

    (Nanyang Technological University)

  • Guofa Cai

    (Nanyang Technological University)

  • Xinran Zhou

    (Nanyang Technological University
    Singapore-HUJ Alliance for Research and Enterprise (SHARE), Nanomaterials for Energy and Water Nexus (NEW), Campus for Research Excellence and Technological Enterprise (CREATE))

  • Sangbaek Park

    (Nanyang Technological University)

  • Jiaqing Xiong

    (Nanyang Technological University)

  • Pooi See Lee

    (Nanyang Technological University
    Singapore-HUJ Alliance for Research and Enterprise (SHARE), Nanomaterials for Energy and Water Nexus (NEW), Campus for Research Excellence and Technological Enterprise (CREATE))

Abstract

Advances in next-generation soft electronic devices rely on the development of highly deformable, healable, and printable energy generators to power these electronics. Development of deformable or wearable energy generators that can simultaneously attain extreme stretchability with superior healability remains a daunting challenge. We address this issue by developing a highly conductive, extremely stretchable, and healable composite based on thermoplastic elastomer with liquid metal and silver flakes as the stretchable conductor for triboelectric nanogenerators. The elastomer is used both as the matrix for the conductor and as the triboelectric layer. The nanogenerator showed a stretchability of 2500% and it recovered its energy-harvesting performance after extreme mechanical damage, due to the supramolecular hydrogen bonding of the thermoplastic elastomer. The composite of the thermoplastic elastomer, liquid metal particles, and silver flakes exhibited an initial conductivity of 6250 S cm−1 and recovered 96.0% of its conductivity after healing.

Suggested Citation

  • Kaushik Parida & Gurunathan Thangavel & Guofa Cai & Xinran Zhou & Sangbaek Park & Jiaqing Xiong & Pooi See Lee, 2019. "Extremely stretchable and self-healing conductor based on thermoplastic elastomer for all-three-dimensional printed triboelectric nanogenerator," Nature Communications, Nature, vol. 10(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:10:y:2019:i:1:d:10.1038_s41467-019-10061-y
    DOI: 10.1038/s41467-019-10061-y
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    Cited by:

    1. Ngoc Thanh Phuong Vo & Tae Uk Nam & Min Woo Jeong & Jun Su Kim & Kyu Ho Jung & Yeongjun Lee & Guorong Ma & Xiaodan Gu & Jeffrey B.-H. Tok & Tae Il Lee & Zhenan Bao & Jin Young Oh, 2024. "Autonomous self-healing supramolecular polymer transistors for skin electronics," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    2. Beibei Shao & Ming-Han Lu & Tai-Chen Wu & Wei-Chen Peng & Tien-Yu Ko & Yung-Chi Hsiao & Jiann-Yeu Chen & Baoquan Sun & Ruiyuan Liu & Ying-Chih Lai, 2024. "Large-area, untethered, metamorphic, and omnidirectionally stretchable multiplexing self-powered triboelectric skins," Nature Communications, Nature, vol. 15(1), pages 1-14, December.
    3. Liang Yue & S. Macrae Montgomery & Xiaohao Sun & Luxia Yu & Yuyang Song & Tsuyoshi Nomura & Masato Tanaka & H. Jerry Qi, 2023. "Single-vat single-cure grayscale digital light processing 3D printing of materials with large property difference and high stretchability," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    4. Patnam, Harishkumarreddy & Dudem, Bhaskar & Graham, Sontyana Adonijah & Yu, Jae Su, 2021. "High-performance and robust triboelectric nanogenerators based on optimal microstructured poly(vinyl alcohol) and poly(vinylidene fluoride) polymers for self-powered electronic applications," Energy, Elsevier, vol. 223(C).
    5. Jian Lv & Gurunathan Thangavel & Yangyang Xin & Dace Gao & Wei Church Poh & Shaohua Chen & Pooi See Lee, 2023. "Printed sustainable elastomeric conductor for soft electronics," Nature Communications, Nature, vol. 14(1), pages 1-14, December.

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