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Phonon-enhanced photothermoelectric effect in SrTiO3 ultra-broadband photodetector

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  • Xiaowei Lu

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Peng Jiang

    (Chinese Academy of Sciences)

  • Xinhe Bao

    (Chinese Academy of Sciences)

Abstract

The self-powered and ultra-broadband photodetectors based on photothermoelectric (PTE) effect are promising for diverse applications such as sensing, environmental monitoring, night vision and astronomy. The sensitivity of PTE photodetectors is determined by the Seebeck coefficient and the rising temperature under illumination. Previous PTE photodetectors mostly rely on traditional thermoelectric materials with Seebeck coefficients in the range of 100 μV K−1, and array structures with multiple units are usually employed to enhance the photodetection performance. Herein, we demonstrate a reduced SrTiO3 (r-STO) based PTE photodetector with sensitivity up to 1.2 V W−1 and broadband spectral response from 325 nm to 10.67 μm. The high performance of r-STO PTE photodetector is attributed to its intrinsic high Seebeck coefficient and phonon-enhanced photoresponse in the long wavelength infrared region. Our results open up a new avenue towards searching for novel PTE materials beyond traditional thermoelectric materials for low-cost and high-performance photodetector at room temperature.

Suggested Citation

  • Xiaowei Lu & Peng Jiang & Xinhe Bao, 2019. "Phonon-enhanced photothermoelectric effect in SrTiO3 ultra-broadband photodetector," Nature Communications, Nature, vol. 10(1), pages 1-7, December.
  • Handle: RePEc:nat:natcom:v:10:y:2019:i:1:d:10.1038_s41467-018-07860-0
    DOI: 10.1038/s41467-018-07860-0
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    Cited by:

    1. Bocheng Lv & Yu Liu & Weidong Wu & Yan Xie & Jia-Lin Zhu & Yang Cao & Wanyun Ma & Ning Yang & Weidong Chu & Yi Jia & Jinquan Wei & Jia-Lin Sun, 2022. "Local large temperature difference and ultra-wideband photothermoelectric response of the silver nanostructure film/carbon nanotube film heterostructure," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    2. Yuxuan Zhang & You Meng & Liqiang Wang & Changyong Lan & Quan Quan & Wei Wang & Zhengxun Lai & Weijun Wang & Yezhan Li & Di Yin & Dengji Li & Pengshan Xie & Dong Chen & Zhe Yang & SenPo Yip & Yang Lu , 2024. "Pulse irradiation synthesis of metal chalcogenides on flexible substrates for enhanced photothermoelectric performance," Nature Communications, Nature, vol. 15(1), pages 1-9, December.

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