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Decay on Cyclic CO 2 Capture Performance of Calcium-Based Sorbents Derived from Wasted Precursors in Multicycles

Author

Listed:
  • Dehong Gong

    (School of Energy and Power Engineering, University of Shanghai for Science and Technology, Shanghai 200093, China
    School of Electrical Engineering, Guizhou University, Guiyang 550025, China)

  • Zhongxiao Zhang

    (School of Energy and Power Engineering, University of Shanghai for Science and Technology, Shanghai 200093, China)

  • Ting Zhao

    (School of Electrical Engineering, Guizhou University, Guiyang 550025, China)

Abstract

In order to obtain the cheap waste calcium-based sorbent, three wasted CaCO 3 precursors, namely carbide slag, chicken eggshells, and analytical reagent-grade calcium carbonate, were selected and prepared at 700 °C to form calcium-based sorbents for CO 2 capture. TGA was used to test the CO 2 uptake performance of each calcium-based sorbent in 20 cycles. To identify the decay mechanism of CO 2 uptake with an increasing number of cycles, all calcium-based sorbents were characterized by using XRF, XRD, and N 2 adsorption. The specific surface area of calcium-based sorbents was used to redefine the formula of cyclic carbonation reactivity decay. The carbonation conversion rate of three calcium-based sorbents exhibited a decreasing trend as the cycle number increased. Chicken eggshells exhibited the most significant decrease rate (over 50% compared with Cycle 1), while carbide slag and analytical reagent-grade calcium carbonate showed a flat linear decline trend. The specific surface area of the samples was used to calculate carbonation conversion for an infinite number of cycles. The carbonation conversion rates of three calcium-based sorbents were estimated to decrease to 0.2898, 0.1455, and 0.3438 mol/mol, respectively, after 100 cycles.

Suggested Citation

  • Dehong Gong & Zhongxiao Zhang & Ting Zhao, 2022. "Decay on Cyclic CO 2 Capture Performance of Calcium-Based Sorbents Derived from Wasted Precursors in Multicycles," Energies, MDPI, vol. 15(9), pages 1-15, May.
    • Handle: RePEc:gam:jeners:v:15:y:2022:i:9:p:3335-:d:808096
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    1. Zhao, Ning & You, Fengqi, 2020. "Can renewable generation, energy storage and energy efficient technologies enable carbon neutral energy transition?," Applied Energy, Elsevier, vol. 279(C).
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