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Photocatalytic CO2 reduction to methanol over bismuth promoted BaTiO3 perovskite nanoparticle catalysts

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  • Dasireddy, Venkata D.B.C.
  • Likozar, Blaž

Abstract

The photocatalytic reduction reactions of CO2 to methanol over bismuth-promoted BaTiO3 chemical photo-catalyst were reported for the first measurement time. Catalysts were prepared via single step deposition precipitation/solution combustion technique. Phases/morphology were characterised by powder X-ray diffraction (XRD)/scanning electron microscopy (SEM). Light absorption spectrum/bandgap energy (Eg) was calculated using ultraviolet–visible (UV–Vis) wavelength diffuse reflectance spectroscopy. The addition of Ba/Bi increased Eg. Comparing materials, synthesised by combusting, the latter showed a surface high basicity/water adsorption. Tests indicated the formation of alcohols. Bi-containing also demonstrated CO. No CH3OH was found for precipitated though. Activity resulted from the synergetic relationship effect between Bi/Ti, caused by the charge transfer mechanism between these component species, strong interaction phenomena and recombination. All were stable for a long temporal period. In the presence of the Ba or Bi metals over titania, the electrons (e–) from TiO2 form an e––hole pair separation, prolonging their decay lifetime. Ba/Bi-based TiO2 presented produced a CH3OH yield of 5.95 μmol gcat−1 h−1, higher compared to structured catalytic systems, described in specific literature reports. As opposed to hydrogen, CH3OH is a renewable storable liquid solar fuel, not only integrating carbon capture and utilisation (CCU), but also power-to-liquid.

Suggested Citation

  • Dasireddy, Venkata D.B.C. & Likozar, Blaž, 2022. "Photocatalytic CO2 reduction to methanol over bismuth promoted BaTiO3 perovskite nanoparticle catalysts," Renewable Energy, Elsevier, vol. 195(C), pages 885-895.
    • Handle: RePEc:eee:renene:v:195:y:2022:i:c:p:885-895
    DOI: 10.1016/j.renene.2022.06.064
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    References listed on IDEAS

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    1. Dasireddy, Venkata D.B.C. & Likozar, Blaž, 2019. "The role of copper oxidation state in Cu/ZnO/Al2O3 catalysts in CO2 hydrogenation and methanol productivity," Renewable Energy, Elsevier, vol. 140(C), pages 452-460.
    2. Jiang, Yuan & Bhattacharyya, Debangsu, 2017. "Techno-economic analysis of direct coal-biomass to liquids (CBTL) plants with shale gas utilization and CO2 capture and storage (CCS)," Applied Energy, Elsevier, vol. 189(C), pages 433-448.
    3. Jingrun Ran & Guoping Gao & Fa-Tang Li & Tian-Yi Ma & Aijun Du & Shi-Zhang Qiao, 2017. "Ti3C2 MXene co-catalyst on metal sulfide photo-absorbers for enhanced visible-light photocatalytic hydrogen production," Nature Communications, Nature, vol. 8(1), pages 1-10, April.
    4. Rahman, Farahiyah Abdul & Aziz, Md Maniruzzaman A. & Saidur, R. & Bakar, Wan Azelee Wan Abu & Hainin, M.R & Putrajaya, Ramadhansyah & Hassan, Norhidayah Abdul, 2017. "Pollution to solution: Capture and sequestration of carbon dioxide (CO2) and its utilization as a renewable energy source for a sustainable future," Renewable and Sustainable Energy Reviews, Elsevier, vol. 71(C), pages 112-126.
    5. Dasireddy, Venkata D.B.C. & Likozar, Blaž, 2022. "Cu–Mn–O nano-particle/nano-sheet spinel-type materials as catalysts in methanol steam reforming (MSR) and preferential oxidation (PROX) reaction for purified hydrogen production," Renewable Energy, Elsevier, vol. 182(C), pages 713-724.
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    1. Pérez-Hernández, Raúl & Martínez, Albina Gutiérrez & Galicia, Gilberto Mondragón & Fernández García, María E. & Nuñez, Oscar Carrera & Hernández, Miriam Vega & López, Pavel & Gutiérrez Wing, Claudia E, 2023. "Carbon cycle using the CO2 conversion to methane as environmental feasibility on Ni/TiO2-Na nanotubes catalysts," Renewable Energy, Elsevier, vol. 217(C).

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