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A coupled lattice Boltzmann model for simulating reactive transport in CO2 injection

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  • Tian, Zhiwei
  • Xing, Huilin
  • Tan, Yunliang
  • Gao, Jinfang

Abstract

A lattice Boltzmann method (LBM) based computational REV model of geochemical reaction is proposed to describe the geochemical reactions of both solute ions transport and solid phase CaCO3 dissolution in CO2-saturated water as well as their effects on the velocity fields of fluid flows during a CO2 injection process. This includes the porosity change with the calcium carbonate dissolution and its feedback impacts on fluid flows. The proposed model is implemented in our in-house LBM code and verified through a hypothetic numerical experiment. The interaction between chemical reactions and fluid advection–diffusion processes is investigated through comparing simulation results of different species distribution at different stages. It has been well known that even a small porosity change induced by the chemical reaction would cause an obvious permeability change. Our present results validate that rule, and furthermore yield a numerical relationship between porosity change and fluid velocity increase at different time steps. This demonstrates that the proposed LBM geochemical reaction model may serve as a reliable approach to investigate the reactive transport in reservoirs of CO2 injection.

Suggested Citation

  • Tian, Zhiwei & Xing, Huilin & Tan, Yunliang & Gao, Jinfang, 2014. "A coupled lattice Boltzmann model for simulating reactive transport in CO2 injection," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 403(C), pages 155-164.
    • Handle: RePEc:eee:phsmap:v:403:y:2014:i:c:p:155-164
    DOI: 10.1016/j.physa.2014.02.040
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    References listed on IDEAS

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    1. Zhi-Wei Tian & Sheng Chen & Chu-Guang Zheng, 2010. "Lattice Boltzmann Simulation Of Gaseous Finite-Knudsen Microflows," International Journal of Modern Physics C (IJMPC), World Scientific Publishing Co. Pte. Ltd., vol. 21(06), pages 769-783.
    2. Zhiwei Tian & Yunliang Tan & Sheng Chen, 2012. "A Numerical Study On Premixed Microcombustion By Lattice Boltzmann Method," International Journal of Modern Physics C (IJMPC), World Scientific Publishing Co. Pte. Ltd., vol. 23(05), pages 1-13.
    3. Tian, Zhi-Wei & Zou, Chun & Liu, Hong-Juan & Guo, Zhao-Li & Liu, Zhao-Hui & Zheng, Chu-Guang, 2007. "Lattice Boltzmann scheme for simulating thermal micro-flow," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 385(1), pages 59-68.
    4. Chen, Sheng & Tian, Zhiwei, 2009. "Simulation of microchannel flow using the lattice Boltzmann method," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 388(23), pages 4803-4810.
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    Cited by:

    1. Yidi Wan & Chengzao Jia & Wen Zhao & Lin Jiang & Zhuxin Chen, 2023. "Micro-Scale Lattice Boltzmann Simulation of Two-Phase CO 2 –Brine Flow in a Tighter REV Extracted from a Permeable Sandstone Core: Implications for CO 2 Storage Efficiency," Energies, MDPI, vol. 16(3), pages 1-26, February.
    2. Zhigao Peng & Shenggui Liu & Yingjun Li & Zongwei Deng & Haoxiong Feng, 2020. "Pore-Scale Lattice Boltzmann Simulation of Gas Diffusion–Adsorption Kinetics Considering Adsorption-Induced Diffusivity Change," Energies, MDPI, vol. 13(18), pages 1-18, September.

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