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Integration of H2-separating membrane technology in gas turbine processes for CO2 capture

Author

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  • Jordal, K.
  • Bredesen, R.
  • Kvamsdal, H.M.
  • Bolland, O.

Abstract

The paper describes the promising possibility to capture CO2 in natural gas fired power cycles through the use of a high-temperature membrane reactor of the methane-steam reforming type with an integrated H2-separating membrane. Two types of membranes are investigated: Pd membranes, which could allow for zero-emission power cycles, and microporous membranes, the use of which in the present work means that 20% of the generated CO2 is emitted to the atmosphere. The membrane reactor is a complex component and much further work is required to find optimum power cycle operating conditions. Combined cycles with an integrated membrane reactor were investigated and the thermal efficiency in some of these non-optimized cases was superior at 47%.

Suggested Citation

  • Jordal, K. & Bredesen, R. & Kvamsdal, H.M. & Bolland, O., 2004. "Integration of H2-separating membrane technology in gas turbine processes for CO2 capture," Energy, Elsevier, vol. 29(9), pages 1269-1278.
    • Handle: RePEc:eee:energy:v:29:y:2004:i:9:p:1269-1278
    DOI: 10.1016/j.energy.2004.03.086
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    1. Sjardin, M. & Damen, K.J. & Faaij, A.P.C., 2006. "Techno-economic prospects of small-scale membrane reactors in a future hydrogen-fuelled transportation sector," Energy, Elsevier, vol. 31(14), pages 2523-2555.
    2. Martínez, I. & Romano, M.C. & Fernández, J.R. & Chiesa, P. & Murillo, R. & Abanades, J.C., 2014. "Process design of a hydrogen production plant from natural gas with CO2 capture based on a novel Ca/Cu chemical loop," Applied Energy, Elsevier, vol. 114(C), pages 192-208.
    3. Zhang, Guoqiang & Li, Yuanyuan & Zhang, Na, 2017. "Performance analysis of a novel low CO2-emission solar hybrid combined cycle power system," Energy, Elsevier, vol. 128(C), pages 152-162.
    4. Fontina Petrakopoulou & Diego Iribarren & Javier Dufour, 2015. "Life‐cycle performance of natural gas power plants with pre‐combustion CO2 capture," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 5(3), pages 268-276, June.
    5. Li, Yuanyuan & Zhang, Na & Cai, Ruixian, 2013. "Low CO2-emissions hybrid solar combined-cycle power system with methane membrane reforming," Energy, Elsevier, vol. 58(C), pages 36-44.
    6. Yang, Ming-Ke & Han, Yu & Zou, En-Bao & Chen, Wan & Peng, Xiao-Wan & Dong, Bao-Can & Sun, Chang-Yu & Liu, Bei & Chen, Guang-Jin, 2020. "Separation of IGCC syngas by using ZIF-8/dimethylacetamide slurry with high CO2 sorption capacity and sorption speed but low sorption heat," Energy, Elsevier, vol. 201(C).

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