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Supramolecular porous-based phase change material based on cucurbit[7]uril complexed amino-montmorillonite

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Listed:
  • Wang, Huihui
  • Zou, Changjun
  • Hu, Yujie
  • Xiong, Tingting
  • Tang, Wenyue

Abstract

Under high-temperature conditions, drill bits, downhole guiding tools, etc. are susceptible to failure, so capturing and storing the heat energy generated is critical for efficient drilling. In this work, a porous material of cucurbit[7]uril (CB[7]) complexed amino-montmorillonite (NH2-MT) was proposed for the first time to encapsulate eutectic nitrate (NIT) to alleviate the high-temperature crisis in the drilling process. The results showed that the structural stability and anti-leakage performance of the supramolecular composite phase change materials (MAC@NIT) were significantly improved by the addition 0.25 g of CB[7], and the adsorption of Na+ and K+ by CB[7] was in the form of monolayer adsorption. The phase change temperature and structure of MAC@NIT-2 remained stable after 200 cycles, and the maximum change of latent heat of solid-liquid was only 3.96 J/g. The special cavity structure of CB[7] further enhanced the thermal conductivity of the MAC@NIT, up to 0.48 W/m·k, which was 20 % higher than the MT@NIT. The addition of MAC@NIT improves the stability of the drilling fluids by 15 %. Additionally, the temperature of the drilling fluids could be reduced by 4.3 °C at a low solid-solid latent heat value. In summary, this study provides ideas for developing ultra-deep oil and gas resources efficiently.

Suggested Citation

  • Wang, Huihui & Zou, Changjun & Hu, Yujie & Xiong, Tingting & Tang, Wenyue, 2024. "Supramolecular porous-based phase change material based on cucurbit[7]uril complexed amino-montmorillonite," Energy, Elsevier, vol. 288(C).
    • Handle: RePEc:eee:energy:v:288:y:2024:i:c:s0360544223031730
    DOI: 10.1016/j.energy.2023.129779
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    References listed on IDEAS

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    1. Xu, J.X. & Li, T.X. & Chao, J.W. & Yan, T.S. & Wang, R.Z., 2019. "High energy-density multi-form thermochemical energy storage based on multi-step sorption processes," Energy, Elsevier, vol. 185(C), pages 1131-1142.
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    3. Zhao, Xin & Geng, Qi & Zhang, Zhen & Qiu, Zhengsong & Fang, Qingchao & Wang, Zhiyuan & Yan, Chuanliang & Ma, Yongle & Li, Yang, 2023. "Phase change material microcapsules for smart temperature regulation of drilling fluids for gas hydrate reservoirs," Energy, Elsevier, vol. 263(PB).
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