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Designed formation of lignin-derived hollow particle-based carbon nanofibers for high-performance supercapacitors

Author

Listed:
  • Zhou, Man
  • Wang, Ping
  • Yu, Yuanyuan
  • Ma, Wujun
  • Cai, Zaisheng
  • Ko, Frank
  • Li, Min
  • Wang, Qiang

Abstract

This work constructs a 1D hollow particle-based carbon nanofibers (HCNFs) derived from Zn-based metal-organic-frameworks (MOFs) particles embedded in biomass-based electrospinning nanofibers as high-performance supercapacitor (SC) electrodes. Abundant mesopores are introduced by the pyrolysis of MOFs, which generates uniformly distributed electrolyte storage pools for a fast electrolyte ions channel. Owing to its uniquely hierarchical pore structure, the derived HCNFs exhibit much enhanced supercapacitive performance. The prepared HCNF-1000 electrode has not only a high specific capacitance (229.6 F g−1 at a current density of 2 A g−1) but also good rate performance (176.8 F g−1 at 10 A g−1, 99.1 F g−1 at 30 A g−1). The two-electrode symmetrical system HCNF-SC has an energy density of 5.1 Wh kg−1 when the power density is 0.5 kW kg−1. HCNF-1000-based solid-state supercapacitor HCNF-FSC shows good electrochemical performance even in different folded states, displaying the potential application value for the development of portable wearable devices.

Suggested Citation

  • Zhou, Man & Wang, Ping & Yu, Yuanyuan & Ma, Wujun & Cai, Zaisheng & Ko, Frank & Li, Min & Wang, Qiang, 2023. "Designed formation of lignin-derived hollow particle-based carbon nanofibers for high-performance supercapacitors," Energy, Elsevier, vol. 278(C).
    • Handle: RePEc:eee:energy:v:278:y:2023:i:c:s036054422301099x
    DOI: 10.1016/j.energy.2023.127705
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    References listed on IDEAS

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    1. Lv, Chunfei & Ma, Xiaojun & Guo, Ranran & Li, Dongna & Hua, Xuewen & Jiang, Tianyu & Li, Hongpeng & Liu, Yang, 2023. "Polypyrrole-decorated hierarchical carbon aerogel from liquefied wood enabling high energy density and capacitance supercapacitor," Energy, Elsevier, vol. 270(C).
    2. Sakthivel, Mani & Ramki, Settu & Chen, Shen-Ming & Ho, Kuo-Chuan, 2022. "Defect rich Se–CoWS2 as anode and banana flower skin-derived activated carbon channels with interconnected porous structure as cathode materials for asymmetric supercapacitor application," Energy, Elsevier, vol. 257(C).
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