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Preparation and properties of PEDOT:PSS/Te nanorod composite films for flexible thermoelectric power generator

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  • Song, Haijun
  • Cai, Kefeng

Abstract

Poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) functionalized Te (PF-Te) nanorods were in situ synthesized. A simple and efficient vacuum-assisted filtration method was employed to integrate the PF-Te nanorods with PEDOT:PSS to form PEDOT:PSS/PF-Te composite films. By varying the content of PF-Te nanorods, the Seebeck coefficient of the composites increases from 15.6 to 51.6 μV/K, while the electrical conductivity decreases from 1262 to 122.4 S/cm. A maximum power factor of 51.4 μW/mK2 is obtained from a sample containing 70 wt% PF-Te nanorods at room temperature. An 8 single-leg flexible thermoelectric generator prototype was fabricated using the as-prepared PEDOT:PSS/PF-Te composite film containing 70 wt% PF-Te on a polyimide substrate with Ag electrodes. The prototype produced an output voltage of 2.5 mV at a 13.4 K temperature difference between human body and the environment.

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  • Song, Haijun & Cai, Kefeng, 2017. "Preparation and properties of PEDOT:PSS/Te nanorod composite films for flexible thermoelectric power generator," Energy, Elsevier, vol. 125(C), pages 519-525.
    • Handle: RePEc:eee:energy:v:125:y:2017:i:c:p:519-525
    DOI: 10.1016/j.energy.2017.01.037
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    References listed on IDEAS

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    1. Fengjiao Zhang & Yaping Zang & Dazhen Huang & Chong-an Di & Daoben Zhu, 2015. "Flexible and self-powered temperature–pressure dual-parameter sensors using microstructure-frame-supported organic thermoelectric materials," Nature Communications, Nature, vol. 6(1), pages 1-10, December.
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    Cited by:

    1. Sarkar, Kamanashis & Debnath, Ajit & Deb, Krishna & Bera, Arun & Saha, Biswajit, 2019. "Effect of NiO incorporation in charge transport of polyaniline: Improved polymer based thermoelectric generator," Energy, Elsevier, vol. 177(C), pages 203-210.
    2. Karalis, George & Tzounis, Lazaros & Mytafides, Christos K. & Tsirka, Kyriaki & Formanek, Petr & Stylianakis, Minas & Kymakis, Emmanuel & Paipetis, Alkiviadis S., 2021. "A high performance flexible and robust printed thermoelectric generator based on hybridized Te nanowires with PEDOT:PSS," Applied Energy, Elsevier, vol. 294(C).
    3. Su, Ning & Zhu, Pengfei & Pan, Yuhui & Li, Fu & Li, Bo, 2020. "3D-printing of shape-controllable thermoelectric devices with enhanced output performance," Energy, Elsevier, vol. 195(C).
    4. Ni, Dan & Song, Haijun & Chen, Yuanxun & Cai, Kefeng, 2019. "Free-standing highly conducting PEDOT films for flexible thermoelectric generator," Energy, Elsevier, vol. 170(C), pages 53-61.
    5. Chen, Siyu & Xue, Yejian & Li, Jianming & Zhang, Houcheng & Zhou, Lihua & Li, Yangyang, 2023. "Efficient and geometry-matching two-stage annular thermoelectric generator for tubular solid oxide fuel cell waste heat recovery," Energy, Elsevier, vol. 285(C).
    6. Hasan, Mohammed Nazibul & Nayan, Nafarizal & Nafea, Marwan & Muthalif, Asan G.A. & Mohamed Ali, Mohamed Sultan, 2022. "Novel structural design of wearable thermoelectric generator with vertically oriented thermoelements," Energy, Elsevier, vol. 259(C).
    7. Zhang, Houcheng & Xu, Haoran & Chen, Bin & Dong, Feifei & Ni, Meng, 2017. "Two-stage thermoelectric generators for waste heat recovery from solid oxide fuel cells," Energy, Elsevier, vol. 132(C), pages 280-288.
    8. Fan, Zeng & Zhang, Yaoyun & Pan, Lujun & Ouyang, Jianyong & Zhang, Qian, 2021. "Recent developments in flexible thermoelectrics: From materials to devices," Renewable and Sustainable Energy Reviews, Elsevier, vol. 137(C).

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