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Electrocatalytic hydrogen evolution reaction on nano-nickel decorated graphene electrode

Author

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  • Mahale, Nilesh K.
  • Ingle, Sopan T.

Abstract

The quest for the replacement of noble metal electrocatalyst for the hydrogen evolution reaction (HER) with lowest overpotential and Tafel slope is still a major challenge. In the present work new concept of earth abundant material like transition metals (Ni) are composed with graphene sheets as a catalyst to increase the rate of hydrogen production. The nickel nanoparticles are decorated uniformly on graphene sheets via electrophoretic deposition (EPD) method to enhance it's HER performance in alkaline solution. The composite is characterized by XRD, FTIR, XPS, SEM and TEM techniques. The composite shown improved HER performance with a low overpotential of 65 mV for 10 mA cm−2, a small Tafel slope of 54 mV dec−1 and longtime stability.

Suggested Citation

  • Mahale, Nilesh K. & Ingle, Sopan T., 2017. "Electrocatalytic hydrogen evolution reaction on nano-nickel decorated graphene electrode," Energy, Elsevier, vol. 119(C), pages 872-878.
    • Handle: RePEc:eee:energy:v:119:y:2017:i:c:p:872-878
    DOI: 10.1016/j.energy.2016.11.053
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    Cited by:

    1. Li, Junyi & Jiang, Jinxia & Zhou, Yiguang & Chen, Mo & Xiao, Shuhao & Niu, Xiaobin & Wu, Rui & Yu, Le & Blackwood, Daniel John & Chen, Jun Song, 2023. "Nickel single-atom catalysts on porous carbon nanosheets for high-performance lithium-selenium batteries," Energy, Elsevier, vol. 285(C).
    2. Singh, Ram Sevak & Jansen, Maurice & Ganguly, Dipsikha & Kulkarni, Giridhar U. & Ramaprabhu, Sundara & Choudhary, Shyam Kumar & Pramanik, Chandrani, 2022. "Shellac derived graphene films on solid, flexible, and porous substrates for high performance bipolar plates and supercapacitor electrodes," Renewable Energy, Elsevier, vol. 181(C), pages 1008-1022.
    3. Liu, Wei & Tan, Wenyu & He, Hanwei & Peng, Yizhi & Chen, Yuxiang & Yang, Yang, 2022. "One–step electrodeposition of Ni–Ce–Pr–Ho/NF as an efficient electrocatalyst for hydrogen evolution reaction in alkaline medium," Energy, Elsevier, vol. 250(C).
    4. Monama, Gobeng R. & Mdluli, Siyabonga B. & Mashao, Gloria & Makhafola, Mogwasha D. & Ramohlola, Kabelo E. & Molapo, Kerileng M. & Hato, Mpitloane J. & Makgopa, Katlego & Iwuoha, Emmanuel I. & Modibane, 2018. "Palladium deposition on copper(II) phthalocyanine/metal organic framework composite and electrocatalytic activity of the modified electrode towards the hydrogen evolution reaction," Renewable Energy, Elsevier, vol. 119(C), pages 62-72.

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