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Fuel from the synthesis gas--the role of process engineering

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  • Stelmachowski, Marek
  • Nowicki, Lech

Abstract

The paper presents the conclusions obtained in the investigations of methanol synthesis, Fischer-Tropsch synthesis, and higher alcohols synthesis from syngas as a raw material in slurry reactors. The overview of the role of process engineering was made on the basis of the experience in optimizing process conditions, modeling reactors and working out new technologies. Experimental data, obtained with a laboratory-stirred autoclave and theoretical considerations were used to develop the kinetic models that can describe the product formation and the model of the simultaneous phase and chemical equilibrium for the methanol and Fischer-Tropsch syntheses in the slurry reactors. These models were employed in modeling of the bubble-column slurry reactor (BCSR). Based on these considerations, a computer simulation of the low-pressure methanol synthesis for the pilot-scale, BCSR, was devised. The results of the calculations and the conclusions could be employed in the process for designing an industrial plant.

Suggested Citation

  • Stelmachowski, Marek & Nowicki, Lech, 2003. "Fuel from the synthesis gas--the role of process engineering," Applied Energy, Elsevier, vol. 74(1-2), pages 85-93, January.
    • Handle: RePEc:eee:appene:v:74:y:2003:i:1-2:p:85-93
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    Citations

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    Cited by:

    1. Srirangan, Kajan & Akawi, Lamees & Moo-Young, Murray & Chou, C. Perry, 2012. "Towards sustainable production of clean energy carriers from biomass resources," Applied Energy, Elsevier, vol. 100(C), pages 172-186.
    2. Antonio Molino & Vincenzo Larocca & Simeone Chianese & Dino Musmarra, 2018. "Biofuels Production by Biomass Gasification: A Review," Energies, MDPI, vol. 11(4), pages 1-31, March.
    3. Ding, Mingyue & Yang, Yong & Li, Yongwang & Wang, Tiejun & Ma, Longlong & Wu, Chuangzhi, 2013. "Impact of H2/CO ratios on phase and performance of Mn-modified Fe-based Fischer Tropsch synthesis catalyst," Applied Energy, Elsevier, vol. 112(C), pages 1241-1246.
    4. Chen, Wei-Hsin & Lin, Bo-Jhih & Lee, How-Ming & Huang, Men-Han, 2012. "One-step synthesis of dimethyl ether from the gas mixture containing CO2 with high space velocity," Applied Energy, Elsevier, vol. 98(C), pages 92-101.
    5. Chen, Wei-Hsin & Lin, Bo-Jhih, 2013. "Hydrogen and synthesis gas production from activated carbon and steam via reusing carbon dioxide," Applied Energy, Elsevier, vol. 101(C), pages 551-559.
    6. Castelo Branco, David A. & Szklo, Alexandre S. & Schaeffer, Roberto, 2010. "Co2e emissions abatement costs of reducing natural gas flaring in Brazil by investing in offshore GTL plants producing premium diesel," Energy, Elsevier, vol. 35(1), pages 158-167.
    7. Khobragade, Murnal & Majhi, Sachchit & Pant, K.K., 2012. "Effect of K and CeO2 promoters on the activity of Co/SiO2 catalyst for liquid fuel production from syngas," Applied Energy, Elsevier, vol. 94(C), pages 385-394.
    8. Ding, Mingyue & Tu, Junling & Qiu, Minghuang & Wang, Tiejun & Ma, Longlong & Li, Yuping, 2015. "Impact of potassium promoter on Cu–Fe based mixed alcohols synthesis catalyst," Applied Energy, Elsevier, vol. 138(C), pages 584-589.
    9. Song, Xueping & Guo, Zhancheng, 2007. "Production of synthesis gas by co-gasifying coke and natural gas in a fixed bed reactor," Energy, Elsevier, vol. 32(10), pages 1972-1978.

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    Keywords

    Fuel Synthesis gas;

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