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Applied kinetics for modeling of reactive hot gas filters

Author

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  • Rhyner, Urs
  • Edinger, Philip
  • Schildhauer, Tilman J.
  • Biollaz, Serge M.A.

Abstract

First order kinetics were developed based on experimental results of a noble metal catalyst. Activation energies and pre-exponential factors were determined by parameter estimation for steam reforming of tars, sulfur tars and ethene. The formation of ethane and benzene was assumed to be at constant rate depending on the decomposition of ethene and toluene respectively. Further, for steam reforming of methane and water gas shift reaction, the kinetic parameters of Langmuir–Hinshelwood–Hougen–Watson (LHHW) type rate laws including equilibrium term and adsorption of sulfur could be determined.

Suggested Citation

  • Rhyner, Urs & Edinger, Philip & Schildhauer, Tilman J. & Biollaz, Serge M.A., 2014. "Applied kinetics for modeling of reactive hot gas filters," Applied Energy, Elsevier, vol. 113(C), pages 766-780.
    • Handle: RePEc:eee:appene:v:113:y:2014:i:c:p:766-780
    DOI: 10.1016/j.apenergy.2013.07.063
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    Cited by:

    1. Hu, Fu-Xiang & Yang, Guo-Hua & Ding, Guo-Zhu & Li, Zhen & Du, Ka-Shuai & Hu, Zhi-Fa & Tian, Su-Rui, 2016. "Experimental study on catalytic cracking of model tar compounds in a dual layer granular bed filter," Applied Energy, Elsevier, vol. 170(C), pages 47-57.
    2. Devin Peck & Mark Zappi & Daniel Gang & John Guillory & Rafael Hernandez & Prashanth Buchireddy, 2023. "Review of Porous Ceramics for Hot Gas Cleanup of Biomass Syngas Using Catalytic Ceramic Filters to Produce Green Hydrogen/Fuels/Chemicals," Energies, MDPI, vol. 16(5), pages 1-32, February.
    3. Li, Xingxing & Zhu, Gangli & Qi, Suitao & Huang, Jun & Yang, Bolun, 2014. "Simultaneous production of hythane and carbon nanotubes via catalytic decomposition of methane with catalysts dispersed on porous supports," Applied Energy, Elsevier, vol. 130(C), pages 846-852.
    4. Yeo, Tze Yuen & Ashok, Jangam & Kawi, Sibudjing, 2019. "Recent developments in sulphur-resilient catalytic systems for syngas production," Renewable and Sustainable Energy Reviews, Elsevier, vol. 100(C), pages 52-70.
    5. Moioli, Emanuele & Schildhauer, Tilman, 2022. "Negative CO2 emissions from flexible biofuel synthesis: Concepts, potentials, technologies," Renewable and Sustainable Energy Reviews, Elsevier, vol. 158(C).

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