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Quantum textures of the many-body wavefunctions in magic-angle graphene

Author

Listed:
  • Kevin P. Nuckolls

    (Princeton University)

  • Ryan L. Lee

    (Princeton University)

  • Myungchul Oh

    (Princeton University)

  • Dillon Wong

    (Princeton University)

  • Tomohiro Soejima

    (University of California)

  • Jung Pyo Hong

    (Princeton University)

  • Dumitru Călugăru

    (Princeton University)

  • Jonah Herzog-Arbeitman

    (Princeton University)

  • B. Andrei Bernevig

    (Princeton University
    Donostia International Physics Center
    IKERBASQUE, Basque Foundation for Science)

  • Kenji Watanabe

    (Research Center for Functional Materials, National Institute for Materials Science)

  • Takashi Taniguchi

    (International Center for Materials Nanoarchitectonics, National Institute for Materials Science)

  • Nicolas Regnault

    (Laboratoire de Physique de l’Ecole normale supérieure, ENS, Université PSL, CNRS, Sorbonne Université, Université Paris-Diderot, Sorbonne Paris Cité)

  • Michael P. Zaletel

    (University of California
    Materials Sciences Division, Lawrence Berkeley National Laboratory)

  • Ali Yazdani

    (Princeton University)

Abstract

Interactions among electrons create novel many-body quantum phases of matter with wavefunctions that reflect electronic correlation effects, broken symmetries and collective excitations. Many quantum phases have been discovered in magic-angle twisted bilayer graphene (MATBG), including correlated insulating1, unconventional superconducting2–5 and magnetic topological6–9 phases. The lack of microscopic information10,11 of possible broken symmetries has hampered our understanding of these phases12–17. Here we use high-resolution scanning tunnelling microscopy to study the wavefunctions of the correlated phases in MATBG. The squares of the wavefunctions of gapped phases, including those of the correlated insulating, pseudogap and superconducting phases, show distinct broken-symmetry patterns with a √3 × √3 super-periodicity on the graphene atomic lattice that has a complex spatial dependence on the moiré scale. We introduce a symmetry-based analysis using a set of complex-valued local order parameters, which show intricate textures that distinguish the various correlated phases. We compare the observed quantum textures of the correlated insulators at fillings of ±2 electrons per moiré unit cell to those expected for proposed theoretical ground states. In typical MATBG devices, these textures closely match those of the proposed incommensurate Kekulé spiral order15, whereas in ultralow-strain samples, our data have local symmetries like those of a time-reversal symmetric intervalley coherent phase12. Moreover, the superconducting state of MATBG shows strong signatures of intervalley coherence, only distinguishable from those of the insulator with our phase-sensitive measurements.

Suggested Citation

  • Kevin P. Nuckolls & Ryan L. Lee & Myungchul Oh & Dillon Wong & Tomohiro Soejima & Jung Pyo Hong & Dumitru Călugăru & Jonah Herzog-Arbeitman & B. Andrei Bernevig & Kenji Watanabe & Takashi Taniguchi & , 2023. "Quantum textures of the many-body wavefunctions in magic-angle graphene," Nature, Nature, vol. 620(7974), pages 525-532, August.
  • Handle: RePEc:nat:nature:v:620:y:2023:i:7974:d:10.1038_s41586-023-06226-x
    DOI: 10.1038/s41586-023-06226-x
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    Cited by:

    1. Maine Christos & Subir Sachdev & Mathias S. Scheurer, 2023. "Nodal band-off-diagonal superconductivity in twisted graphene superlattices," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    2. Yifei Guan & Clement Dutreix & Héctor González-Herrero & Miguel M. Ugeda & Ivan Brihuega & Mikhail I. Katsnelson & Oleg V. Yazyev & Vincent T. Renard, 2024. "Observation of Kekulé vortices around hydrogen adatoms in graphene," Nature Communications, Nature, vol. 15(1), pages 1-6, December.
    3. Jesse C. Hoke & Yifan Li & Julian May-Mann & Kenji Watanabe & Takashi Taniguchi & Barry Bradlyn & Taylor L. Hughes & Benjamin E. Feldman, 2024. "Uncovering the spin ordering in magic-angle graphene via edge state equilibration," Nature Communications, Nature, vol. 15(1), pages 1-7, December.

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