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Topologically protected magnetoelectric switching in a multiferroic

Author

Listed:
  • Louis Ponet

    (Istituto Italiano di Tecnologia
    Scuola Normale Superiore di Pisa
    École Polytechnique Fédérale de Lausanne)

  • S. Artyukhin

    (Istituto Italiano di Tecnologia)

  • Th. Kain

    (Vienna University of Technology)

  • J. Wettstein

    (Vienna University of Technology)

  • Anna Pimenov

    (Vienna University of Technology)

  • A. Shuvaev

    (Vienna University of Technology)

  • X. Wang

    (Beijing Institute of Technology
    Rutgers Center for Emergent Materials and Department of Physics and Astronomy)

  • S.-W. Cheong

    (Rutgers Center for Emergent Materials and Department of Physics and Astronomy)

  • Maxim Mostovoy

    (University of Groningen)

  • Andrei Pimenov

    (Vienna University of Technology)

Abstract

Electric control of magnetism and magnetic control of ferroelectricity can improve the energy efficiency of magnetic memory and data-processing devices1. However, the necessary magnetoelectric switching is hard to achieve, and requires more than just a coupling between the spin and the charge degrees of freedom2–5. Here we show that an application and subsequent removal of a magnetic field reverses the electric polarization of the multiferroic GdMn2O5, thus requiring two cycles to bring the system back to the original configuration. During this unusual hysteresis loop, four states with different magnetic configurations are visited by the system, with one half of all spins undergoing unidirectional full-circle rotation in increments of about 90 degrees. Therefore, GdMn2O5 acts as a magnetic crankshaft that converts the back-and-forth variations of the magnetic field into a circular spin motion. This peculiar four-state magnetoelectric switching emerges as a topologically protected boundary between different two-state switching regimes. Our findings establish a paradigm of topologically protected switching phenomena in ferroic materials.

Suggested Citation

  • Louis Ponet & S. Artyukhin & Th. Kain & J. Wettstein & Anna Pimenov & A. Shuvaev & X. Wang & S.-W. Cheong & Maxim Mostovoy & Andrei Pimenov, 2022. "Topologically protected magnetoelectric switching in a multiferroic," Nature, Nature, vol. 607(7917), pages 81-85, July.
  • Handle: RePEc:nat:nature:v:607:y:2022:i:7917:d:10.1038_s41586-022-04851-6
    DOI: 10.1038/s41586-022-04851-6
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    Cited by:

    1. Yangliu Wu & Zhaozhuo Zeng & Haipeng Lu & Xiaocang Han & Chendi Yang & Nanshu Liu & Xiaoxu Zhao & Liang Qiao & Wei Ji & Renchao Che & Longjiang Deng & Peng Yan & Bo Peng, 2024. "Coexistence of ferroelectricity and antiferroelectricity in 2D van der Waals multiferroic," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    2. Nan Zhang & Wencong Sun & Yao Zhang & Huan-Huan Jiang & Ren-Gen Xiong & Shuai Dong & Han-Yue Zhang, 2023. "Organic radical ferroelectric crystals with martensitic phase transition," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    3. Makiko Ogino & Yoshihiro Okamura & Kosuke Fujiwara & Takahiro Morimoto & Naoto Nagaosa & Yoshio Kaneko & Yoshinori Tokura & Youtarou Takahashi, 2024. "Terahertz photon to dc current conversion via magnetic excitations of multiferroics," Nature Communications, Nature, vol. 15(1), pages 1-7, December.

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