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Quantum criticality in twisted transition metal dichalcogenides

Author

Listed:
  • Augusto Ghiotto

    (Columbia University)

  • En-Min Shih

    (Columbia University)

  • Giancarlo S. S. G. Pereira

    (Columbia University)

  • Daniel A. Rhodes

    (Columbia University)

  • Bumho Kim

    (Columbia University)

  • Jiawei Zang

    (Columbia University)

  • Andrew J. Millis

    (Columbia University
    Flatiron Institute)

  • Kenji Watanabe

    (National Institute for Materials Science)

  • Takashi Taniguchi

    (National Institute for Materials Science)

  • James C. Hone

    (Columbia University)

  • Lei Wang

    (Columbia University
    Nanjing University)

  • Cory R. Dean

    (Columbia University)

  • Abhay N. Pasupathy

    (Columbia University
    Brookhaven National Laboratory)

Abstract

Near the boundary between ordered and disordered quantum phases, several experiments have demonstrated metallic behaviour that defies the Landau Fermi paradigm1–5. In moiré heterostructures, gate-tuneable insulating phases driven by electronic correlations have been recently discovered6–23. Here, we use transport measurements to characterize metal–insulator transitions (MITs) in twisted WSe2 near half filling of the first moiré subband. We find that the MIT as a function of both density and displacement field is continuous. At the metal–insulator boundary, the resistivity displays strange metal behaviour at low temperatures, with dissipation comparable to that at the Planckian limit. Further into the metallic phase, Fermi liquid behaviour is recovered at low temperature, and this evolves into a quantum critical fan at intermediate temperatures, before eventually reaching an anomalous saturated regime near room temperature. An analysis of the residual resistivity indicates the presence of strong quantum fluctuations in the insulating phase. These results establish twisted WSe2 as a new platform to study doping and bandwidth-controlled metal–insulator quantum phase transitions on the triangular lattice.

Suggested Citation

  • Augusto Ghiotto & En-Min Shih & Giancarlo S. S. G. Pereira & Daniel A. Rhodes & Bumho Kim & Jiawei Zang & Andrew J. Millis & Kenji Watanabe & Takashi Taniguchi & James C. Hone & Lei Wang & Cory R. Dea, 2021. "Quantum criticality in twisted transition metal dichalcogenides," Nature, Nature, vol. 597(7876), pages 345-349, September.
  • Handle: RePEc:nat:nature:v:597:y:2021:i:7876:d:10.1038_s41586-021-03815-6
    DOI: 10.1038/s41586-021-03815-6
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    Cited by:

    1. Binjie Zheng & Junzhuan Wang & Qianghua Wang & Xin Su & Tianye Huang & Songlin Li & Fengqiu Wang & Yi Shi & Xiaomu Wang, 2022. "Quantum criticality of excitonic Mott metal-insulator transitions in black phosphorus," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    2. Beini Gao & Daniel G. Suárez-Forero & Supratik Sarkar & Tsung-Sheng Huang & Deric Session & Mahmoud Jalali Mehrabad & Ruihao Ni & Ming Xie & Pranshoo Upadhyay & Jonathan Vannucci & Sunil Mittal & Kenj, 2024. "Excitonic Mott insulator in a Bose-Fermi-Hubbard system of moiré WS2/WSe2 heterobilayer," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    3. Zhen Lian & Dongxue Chen & Yuze Meng & Xiaotong Chen & Ying Su & Rounak Banerjee & Takashi Taniguchi & Kenji Watanabe & Sefaattin Tongay & Chuanwei Zhang & Yong-Tao Cui & Su-Fei Shi, 2023. "Exciton Superposition across Moiré States in a Semiconducting Moiré Superlattice," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    4. Dorri Halbertal & Simon Turkel & Christopher J. Ciccarino & Jonas B. Profe & Nathan Finney & Valerie Hsieh & Kenji Watanabe & Takashi Taniguchi & James Hone & Cory Dean & Prineha Narang & Abhay N. Pas, 2022. "Unconventional non-local relaxation dynamics in a twisted trilayer graphene moiré superlattice," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    5. Zhen Lian & Dongxue Chen & Lei Ma & Yuze Meng & Ying Su & Li Yan & Xiong Huang & Qiran Wu & Xinyue Chen & Mark Blei & Takashi Taniguchi & Kenji Watanabe & Sefaattin Tongay & Chuanwei Zhang & Yong-Tao , 2023. "Quadrupolar excitons and hybridized interlayer Mott insulator in a trilayer moiré superlattice," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    6. Yanhao Tang & Jie Gu & Song Liu & Kenji Watanabe & Takashi Taniguchi & James C. Hone & Kin Fai Mak & Jie Shan, 2022. "Dielectric catastrophe at the Wigner-Mott transition in a moiré superlattice," Nature Communications, Nature, vol. 13(1), pages 1-7, December.

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