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Visualizing coherent intermolecular dipole–dipole coupling in real space

Author

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  • Yang Zhang

    (Hefei National Laboratory for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China)

  • Yang Luo

    (Hefei National Laboratory for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China)

  • Yao Zhang

    (Hefei National Laboratory for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China)

  • Yun-Jie Yu

    (Hefei National Laboratory for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China)

  • Yan-Min Kuang

    (Hefei National Laboratory for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China)

  • Li Zhang

    (Hefei National Laboratory for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China)

  • Qiu-Shi Meng

    (Hefei National Laboratory for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China)

  • Yi Luo

    (Hefei National Laboratory for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China)

  • Jin-Long Yang

    (Hefei National Laboratory for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China)

  • Zhen-Chao Dong

    (Hefei National Laboratory for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China)

  • J. G. Hou

    (Hefei National Laboratory for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China)

Abstract

Luminescence induced by highly localized excitations that are produced by electrons tunnelling from the tip of a scanning tunnelling microscope is used to map the spatial distribution of the excitonic coupling in well-defined arrangements of a few zinc-phthalocyanine molecules and the dependence of this spatial distribution on the relative orientation and phase of the transition dipoles of the individual molecules.

Suggested Citation

  • Yang Zhang & Yang Luo & Yao Zhang & Yun-Jie Yu & Yan-Min Kuang & Li Zhang & Qiu-Shi Meng & Yi Luo & Jin-Long Yang & Zhen-Chao Dong & J. G. Hou, 2016. "Visualizing coherent intermolecular dipole–dipole coupling in real space," Nature, Nature, vol. 531(7596), pages 623-627, March.
    • Handle: RePEc:nat:nature:v:531:y:2016:i:7596:d:10.1038_nature17428
    DOI: 10.1038/nature17428
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    Citations

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    Cited by:

    1. Jiří Doležal & Sofia Canola & Prokop Hapala & Rodrigo Cezar Campos Ferreira & Pablo Merino & Martin Švec, 2022. "Evidence of exciton-libron coupling in chirally adsorbed single molecules," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    2. Xin Wang & Boyan Liu & Siqing Ma & Yingjuan Zhang & Lianzhou Wang & Gangqiang Zhu & Wei Huang & Songcan Wang, 2024. "Induced dipole moments in amorphous ZnCdS catalysts facilitate photocatalytic H2 evolution," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    3. Yang Luo & Fan-Fang Kong & Xiao-Jun Tian & Yun-Jie Yu & Shi-Hao Jing & Chao Zhang & Gong Chen & Yang Zhang & Yao Zhang & Xiao-Guang Li & Zhen-Yu Zhang & Zhen-Chao Dong, 2024. "Anomalously bright single-molecule upconversion electroluminescence," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    4. Vibhuti Rai & Nico Balzer & Gabriel Derenbach & Christof Holzer & Marcel Mayor & Wulf Wulfhekel & Lukas Gerhard & Michal Valášek, 2023. "Hot luminescence from single-molecule chromophores electrically and mechanically self-decoupled by tripodal scaffolds," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    5. Kirill Vasilev & Benjamin Doppagne & Tomáš Neuman & Anna Rosławska & Hervé Bulou & Alex Boeglin & Fabrice Scheurer & Guillaume Schull, 2022. "Internal Stark effect of single-molecule fluorescence," Nature Communications, Nature, vol. 13(1), pages 1-8, December.

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