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Tracking excited-state charge and spin dynamics in iron coordination complexes

Author

Listed:
  • Wenkai Zhang

    (PULSE Institute, SLAC National Accelerator Laboratory, Stanford University)

  • Roberto Alonso-Mori

    (LCLS, SLAC National Accelerator Laboratory)

  • Uwe Bergmann

    (LCLS, SLAC National Accelerator Laboratory)

  • Christian Bressler

    (European XFEL, D-22761 Hamburg, Germany)

  • Matthieu Chollet

    (LCLS, SLAC National Accelerator Laboratory)

  • Andreas Galler

    (European XFEL, D-22761 Hamburg, Germany)

  • Wojciech Gawelda

    (European XFEL, D-22761 Hamburg, Germany)

  • Ryan G. Hadt

    (Stanford University)

  • Robert W. Hartsock

    (PULSE Institute, SLAC National Accelerator Laboratory, Stanford University
    Stanford University)

  • Thomas Kroll

    (Stanford University)

  • Kasper S. Kjær

    (Centre for Molecular Movies, Niels Bohr Institute, University of Copenhagen, DK-2100 Copenhagen, Denmark
    Centre for Molecular Movies, Technical University of Denmark, DK-2800 Lyngby, Denmark)

  • Katharina Kubiček

    (Max Planck Institute for Biophysical Chemistry, 37077 Göttingen, Germany
    Deutsches Elektronen Synchrotron, Notkestraße 85, 22607 Hamburg, Germany)

  • Henrik T. Lemke

    (LCLS, SLAC National Accelerator Laboratory)

  • Huiyang W. Liang

    (PULSE Institute, SLAC National Accelerator Laboratory, Stanford University
    Stanford University)

  • Drew A. Meyer

    (PULSE Institute, SLAC National Accelerator Laboratory, Stanford University
    Stanford University)

  • Martin M. Nielsen

    (Centre for Molecular Movies, Technical University of Denmark, DK-2800 Lyngby, Denmark)

  • Carola Purser

    (PULSE Institute, SLAC National Accelerator Laboratory, Stanford University)

  • Joseph S. Robinson

    (LCLS, SLAC National Accelerator Laboratory)

  • Edward I. Solomon

    (Stanford University
    SSRL, SLAC National Accelerator Laboratory)

  • Zheng Sun

    (PULSE Institute, SLAC National Accelerator Laboratory, Stanford University)

  • Dimosthenis Sokaras

    (SSRL, SLAC National Accelerator Laboratory)

  • Tim B. van Driel

    (Centre for Molecular Movies, Technical University of Denmark, DK-2800 Lyngby, Denmark)

  • György Vankó

    (Wigner Research Centre for Physics, Hungarian Academy of Sciences, H-1525 Budapest, Hungary)

  • Tsu-Chien Weng

    (SSRL, SLAC National Accelerator Laboratory)

  • Diling Zhu

    (LCLS, SLAC National Accelerator Laboratory)

  • Kelly J. Gaffney

    (PULSE Institute, SLAC National Accelerator Laboratory, Stanford University)

Abstract

Femtosecond resolution X-ray fluorescence spectroscopy is shown to track the charge and spin dynamics triggered when an iron coordination complex is excited by light, and establishes the critical role of intermediate spin states in the de-excitation process.

Suggested Citation

  • Wenkai Zhang & Roberto Alonso-Mori & Uwe Bergmann & Christian Bressler & Matthieu Chollet & Andreas Galler & Wojciech Gawelda & Ryan G. Hadt & Robert W. Hartsock & Thomas Kroll & Kasper S. Kjær & Kath, 2014. "Tracking excited-state charge and spin dynamics in iron coordination complexes," Nature, Nature, vol. 509(7500), pages 345-348, May.
    • Handle: RePEc:nat:nature:v:509:y:2014:i:7500:d:10.1038_nature13252
    DOI: 10.1038/nature13252
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    Cited by:

    1. Marco Reinhard & Alessandro Gallo & Meiyuan Guo & Angel T. Garcia-Esparza & Elisa Biasin & Muhammad Qureshi & Alexander Britz & Kathryn Ledbetter & Kristjan Kunnus & Clemens Weninger & Tim Driel & Jos, 2023. "Ferricyanide photo-aquation pathway revealed by combined femtosecond Kβ main line and valence-to-core x-ray emission spectroscopy," Nature Communications, Nature, vol. 14(1), pages 1-11, December.

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