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Low-temperature aqueous-phase methanol dehydrogenation to hydrogen and carbon dioxide

Author

Listed:
  • Martin Nielsen

    (Leibniz-Institut für Katalyse Eingetragener Verein an der Universität Rostock, Albert-Einstein Straße 29a)

  • Elisabetta Alberico

    (Leibniz-Institut für Katalyse Eingetragener Verein an der Universität Rostock, Albert-Einstein Straße 29a
    Istituto di Chimica Biomolecolare, CNR, traversa La Crucca 3, Sassari 07040, Italy)

  • Wolfgang Baumann

    (Leibniz-Institut für Katalyse Eingetragener Verein an der Universität Rostock, Albert-Einstein Straße 29a)

  • Hans-Joachim Drexler

    (Leibniz-Institut für Katalyse Eingetragener Verein an der Universität Rostock, Albert-Einstein Straße 29a)

  • Henrik Junge

    (Leibniz-Institut für Katalyse Eingetragener Verein an der Universität Rostock, Albert-Einstein Straße 29a)

  • Serafino Gladiali

    (Universitá di Sassari)

  • Matthias Beller

    (Leibniz-Institut für Katalyse Eingetragener Verein an der Universität Rostock, Albert-Einstein Straße 29a)

Abstract

An efficient, low-temperature, aqueous-phase method of producing hydrogen gas from methanol using ruthenium complexes is described, which could make the transport of hydrogen — and hence its use for clean-energy generation — feasible.

Suggested Citation

  • Martin Nielsen & Elisabetta Alberico & Wolfgang Baumann & Hans-Joachim Drexler & Henrik Junge & Serafino Gladiali & Matthias Beller, 2013. "Low-temperature aqueous-phase methanol dehydrogenation to hydrogen and carbon dioxide," Nature, Nature, vol. 495(7439), pages 85-89, March.
    • Handle: RePEc:nat:nature:v:495:y:2013:i:7439:d:10.1038_nature11891
    DOI: 10.1038/nature11891
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    Citations

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    Cited by:

    1. Sai Zhang & Yuxuan Liu & Mingkai Zhang & Yuanyuan Ma & Jun Hu & Yongquan Qu, 2022. "Sustainable production of hydrogen with high purity from methanol and water at low temperatures," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    2. Song, Hongqing & Lao, Junming & Zhang, Liyuan & Xie, Chiyu & Wang, Yuhe, 2023. "Underground hydrogen storage in reservoirs: pore-scale mechanisms and optimization of storage capacity and efficiency," Applied Energy, Elsevier, vol. 337(C).
    3. Zhu, Yong-Qiang & Song, Wei & Wang, Han-Bing & Qi, Jian-Tao & Zeng, Rong-Chang & Ren, Hao & Jiang, Wen-Chun & Meng, Hui-Bo & Li, Yu-Xing, 2024. "Advances in reducing hydrogen effect of pipeline steels on hydrogen-blended natural gas transportation: A systematic review of mitigation strategies," Renewable and Sustainable Energy Reviews, Elsevier, vol. 189(PA).
    4. Wenxuan Xue & Conghui Tang, 2022. "Hydrogenation of CO 2 or CO 2 Derivatives to Methanol under Molecular Catalysis: A Review," Energies, MDPI, vol. 15(6), pages 1-14, March.
    5. Yaguang Li & Xianhua Bai & Dachao Yuan & Fengyu Zhang & Bo Li & Xingyuan San & Baolai Liang & Shufang Wang & Jun Luo & Guangsheng Fu, 2022. "General heterostructure strategy of photothermal materials for scalable solar-heating hydrogen production without the consumption of artificial energy," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    6. Luning Chen & Pragya Verma & Kaipeng Hou & Zhiyuan Qi & Shuchen Zhang & Yi-Sheng Liu & Jinghua Guo & Vitalie Stavila & Mark D. Allendorf & Lansun Zheng & Miquel Salmeron & David Prendergast & Gabor A., 2022. "Reversible dehydrogenation and rehydrogenation of cyclohexane and methylcyclohexane by single-site platinum catalyst," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    7. Hoang, Anh Tuan & Pandey, Ashok & Martinez De Osés, Francisco Javier & Chen, Wei-Hsin & Said, Zafar & Ng, Kim Hoong & Ağbulut, Ümit & Tarełko, Wiesław & Ölçer, Aykut I. & Nguyen, Xuan Phuong, 2023. "Technological solutions for boosting hydrogen role in decarbonization strategies and net-zero goals of world shipping: Challenges and perspectives," Renewable and Sustainable Energy Reviews, Elsevier, vol. 188(C).
    8. Pérez-Fortes, Mar & Schöneberger, Jan C. & Boulamanti, Aikaterini & Tzimas, Evangelos, 2016. "Methanol synthesis using captured CO2 as raw material: Techno-economic and environmental assessment," Applied Energy, Elsevier, vol. 161(C), pages 718-732.

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