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Fractionalized excitations in the spin-liquid state of a kagome-lattice antiferromagnet

Author

Listed:
  • Tian-Heng Han

    (Massachusetts Institute of Technology)

  • Joel S. Helton

    (NIST Center for Neutron Research, National Institute of Standards and Technology)

  • Shaoyan Chu

    (Center for Materials Science and Engineering, Massachusetts Institute of Technology)

  • Daniel G. Nocera

    (Massachusetts Institute of Technology)

  • Jose A. Rodriguez-Rivera

    (NIST Center for Neutron Research, National Institute of Standards and Technology
    University of Maryland, College Park)

  • Collin Broholm

    (NIST Center for Neutron Research, National Institute of Standards and Technology
    The Johns Hopkins University)

  • Young S. Lee

    (Massachusetts Institute of Technology)

Abstract

Neutron scattering measurements on single-crystal samples of the mineral herbertsmithite, which is a spin-1/2 kagome-lattice antiferromagnet, provide evidence of fractionalized spin excitations at low temperatures, indicating that the ground state of herbertsmithite may be a quantum spin liquid.

Suggested Citation

  • Tian-Heng Han & Joel S. Helton & Shaoyan Chu & Daniel G. Nocera & Jose A. Rodriguez-Rivera & Collin Broholm & Young S. Lee, 2012. "Fractionalized excitations in the spin-liquid state of a kagome-lattice antiferromagnet," Nature, Nature, vol. 492(7429), pages 406-410, December.
  • Handle: RePEc:nat:nature:v:492:y:2012:i:7429:d:10.1038_nature11659
    DOI: 10.1038/nature11659
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    Cited by:

    1. Zhicheng Jiang & Zhengtai Liu & Haiyang Ma & Wei Xia & Zhonghao Liu & Jishan Liu & Soohyun Cho & Yichen Yang & Jianyang Ding & Jiayu Liu & Zhe Huang & Yuxi Qiao & Jiajia Shen & Wenchuan Jing & Xiangqi, 2023. "Flat bands, non-trivial band topology and rotation symmetry breaking in layered kagome-lattice RbTi3Bi5," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    2. Yong Hu & Junzhang Ma & Yinxiang Li & Yuxiao Jiang & Dariusz Jakub Gawryluk & Tianchen Hu & Jérémie Teyssier & Volodymyr Multian & Zhouyi Yin & Shuxiang Xu & Soohyeon Shin & Igor Plokhikh & Xinloong H, 2024. "Phonon promoted charge density wave in topological kagome metal ScV6Sn6," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    3. D. Subires & A. Korshunov & A. H. Said & L. Sánchez & Brenden R. Ortiz & Stephen D. Wilson & A. Bosak & S. Blanco-Canosa, 2023. "Order-disorder charge density wave instability in the kagome metal (Cs,Rb)V3Sb5," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    4. Gan Liu & Xinran Ma & Kuanyu He & Qing Li & Hengxin Tan & Yizhou Liu & Jie Xu & Wenna Tang & Kenji Watanabe & Takashi Taniguchi & Libo Gao & Yaomin Dai & Hai-Hu Wen & Binghai Yan & Xiaoxiang Xi, 2022. "Observation of anomalous amplitude modes in the kagome metal CsV3Sb5," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    5. Subhasis Samanta & Hwiwoo Park & Chanhyeon Lee & Sungmin Jeon & Hengbo Cui & Yong-Xin Yao & Jungseek Hwang & Kwang-Yong Choi & Heung-Sik Kim, 2024. "Emergence of flat bands and ferromagnetic fluctuations via orbital-selective electron correlations in Mn-based kagome metal," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    6. Boqin Song & Tianping Ying & Xianxin Wu & Wei Xia & Qiangwei Yin & Qinghua Zhang & Yanpeng Song & Xiaofan Yang & Jiangang Guo & Lin Gu & Xiaolong Chen & Jiangping Hu & Andreas P. Schnyder & Hechang Le, 2023. "Anomalous enhancement of charge density wave in kagome superconductor CsV3Sb5 approaching the 2D limit," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    7. Schmidt, M. & Zimmer, F.M. & Magalhaes, S.G., 2015. "Spin glass induced by infinitesimal disorder in geometrically frustrated kagome lattice," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 438(C), pages 416-423.
    8. Yong Hu & Xianxin Wu & Brenden R. Ortiz & Sailong Ju & Xinloong Han & Junzhang Ma & Nicholas C. Plumb & Milan Radovic & Ronny Thomale & Stephen D. Wilson & Andreas P. Schnyder & Ming Shi, 2022. "Rich nature of Van Hove singularities in Kagome superconductor CsV3Sb5," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    9. Saizheng Cao & Chenchao Xu & Hiroshi Fukui & Taishun Manjo & Ying Dong & Ming Shi & Yang Liu & Chao Cao & Yu Song, 2023. "Competing charge-density wave instabilities in the kagome metal ScV6Sn6," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    10. Sen Zhou & Ziqiang Wang, 2022. "Chern Fermi pocket, topological pair density wave, and charge-4e and charge-6e superconductivity in kagomé superconductors," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    11. Laëtitia Farinacci & Gaël Reecht & Felix Oppen & Katharina J. Franke, 2024. "Yu-Shiba-Rusinov bands in a self-assembled kagome lattice of magnetic molecules," Nature Communications, Nature, vol. 15(1), pages 1-8, December.

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