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Unconventional critical behaviour in a quasi-two-dimensional organic conductor

Author

Listed:
  • F. Kagawa

    (University of Tokyo)

  • K. Miyagawa

    (University of Tokyo
    CREST, Japan Science and Technology Corporation)

  • K. Kanoda

    (University of Tokyo
    CREST, Japan Science and Technology Corporation)

Abstract

Changing the interactions between particles in an ensemble—by varying the temperature or pressure, for example—can lead to phase transitions whose critical behaviour depends on the collective nature of the many-body system. Despite the diversity of ingredients, which include atoms, molecules, electrons and their spins, the collective behaviour can be grouped into several families (called ‘universality classes’) represented by canonical spin models1. One kind of transition, the Mott transition2, occurs when the repulsive Coulomb interaction between electrons is increased, causing wave-like electrons to behave as particles. In two dimensions, the attractive behaviour responsible for the superconductivity in high-transition temperature copper oxide3,4 and organic5,6,7 compounds appears near the Mott transition, but the universality class to which two-dimensional, repulsive electronic systems belongs remains unknown. Here we present an observation of the critical phenomena at the pressure-induced Mott transition in a quasi-two-dimensional organic conductor using conductance measurements as a probe. We find that the Mott transition in two dimensions is not consistent with known universality classes, as the observed collective behaviour has previously not been seen. This peculiarity must be involved in any emergent behaviour near the Mott transition in two dimensions.

Suggested Citation

  • F. Kagawa & K. Miyagawa & K. Kanoda, 2005. "Unconventional critical behaviour in a quasi-two-dimensional organic conductor," Nature, Nature, vol. 436(7050), pages 534-537, July.
  • Handle: RePEc:nat:nature:v:436:y:2005:i:7050:d:10.1038_nature03806
    DOI: 10.1038/nature03806
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    Cited by:

    1. Ye Yang & Fanghang Yu & Xikai Wen & Zhigang Gui & Yuqing Zhang & Fangyang Zhan & Rui Wang & Jianjun Ying & Xianhui Chen, 2023. "Pressure-induced transition from a Mott insulator to a ferromagnetic Weyl metal in La2O3Fe2Se2," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    2. K. Wakamatsu & Y. Suzuki & T. Fujii & K. Miyagawa & H. Taniguchi & K. Kanoda, 2023. "Thermoelectric signature of quantum critical phase in a doped spin-liquid candidate," Nature Communications, Nature, vol. 14(1), pages 1-6, December.

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