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Magnetic control of ferroelectric polarization

Author

Listed:
  • T. Kimura

    (University of Tokyo
    Los Alamos National Laboratory,)

  • T. Goto

    (University of Tokyo)

  • H. Shintani

    (University of Tokyo)

  • K. Ishizaka

    (University of Tokyo)

  • T. Arima

    (University of Tsukuba)

  • Y. Tokura

    (University of Tokyo)

Abstract

The magnetoelectric effect—the induction of magnetization by means of an electric field and induction of polarization by means of a magnetic field—was first presumed to exist by Pierre Curie1, and subsequently attracted a great deal of interest in the 1960s and 1970s (refs 2–4). More recently, related studies on magnetic ferroelectrics5,6,7,8,9,10,11,12,13,14 have signalled a revival of interest in this phenomenon. From a technological point of view, the mutual control of electric and magnetic properties is an attractive possibility15, but the number of candidate materials is limited and the effects are typically too small to be useful in applications. Here we report the discovery of ferroelectricity in a perovskite manganite, TbMnO3, where the effect of spin frustration causes sinusoidal antiferromagnetic ordering. The modulated magnetic structure is accompanied by a magnetoelastically induced lattice modulation, and with the emergence of a spontaneous polarization. In the magnetic ferroelectric TbMnO3, we found gigantic magnetoelectric and magnetocapacitance effects, which can be attributed to switching of the electric polarization induced by magnetic fields. Frustrated spin systems therefore provide a new area to search for magnetoelectric media.

Suggested Citation

  • T. Kimura & T. Goto & H. Shintani & K. Ishizaka & T. Arima & Y. Tokura, 2003. "Magnetic control of ferroelectric polarization," Nature, Nature, vol. 426(6962), pages 55-58, November.
    • Handle: RePEc:nat:nature:v:426:y:2003:i:6962:d:10.1038_nature02018
    DOI: 10.1038/nature02018
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    Cited by:

    1. Shingo Toyoda & Manfred Fiebig & Lea Forster & Taka-hisa Arima & Yoshinori Tokura & Naoki Ogawa, 2021. "Writing of strain-controlled multiferroic ribbons into MnWO4," Nature Communications, Nature, vol. 12(1), pages 1-6, December.
    2. Leixin Miao & Kishwar-E Hasin & Parivash Moradifar & Debangshu Mukherjee & Ke Wang & Sang-Wook Cheong & Elizabeth A. Nowadnick & Nasim Alem, 2022. "Double-Bilayer polar nanoregions and Mn antisites in (Ca, Sr)3Mn2O7," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    3. Qifeng Hu & Yuqiang Huang & Yang Wang & Sujuan Ding & Minjie Zhang & Chenqiang Hua & Linjun Li & Xiangfan Xu & Jinbo Yang & Shengjun Yuan & Kenji Watanabe & Takashi Taniguchi & Yunhao Lu & Chuanhong J, 2024. "Ferrielectricity controlled widely-tunable magnetoelectric coupling in van der Waals multiferroics," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    4. Yangliu Wu & Zhaozhuo Zeng & Haipeng Lu & Xiaocang Han & Chendi Yang & Nanshu Liu & Xiaoxu Zhao & Liang Qiao & Wei Ji & Renchao Che & Longjiang Deng & Peng Yan & Bo Peng, 2024. "Coexistence of ferroelectricity and antiferroelectricity in 2D van der Waals multiferroic," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    5. Yuewen Gao & Toshiaki Iitaka & Zhi Li, 2021. "Terahertz nonlinear optics of chiral semimetals RhSn, HfSn, and PdGa," The European Physical Journal B: Condensed Matter and Complex Systems, Springer;EDP Sciences, vol. 94(5), pages 1-6, May.
    6. Shuai Xu & Jiesu Wang & Pan Chen & Kuijuan Jin & Cheng Ma & Shiyao Wu & Erjia Guo & Chen Ge & Can Wang & Xiulai Xu & Hongbao Yao & Jingyi Wang & Donggang Xie & Xinyan Wang & Kai Chang & Xuedong Bai & , 2023. "Magnetoelectric coupling in multiferroics probed by optical second harmonic generation," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    7. S. Iguchi & R. Masuda & S. Seki & Y. Tokura & Y. Takahashi, 2021. "Enhanced gyrotropic birefringence and natural optical activity on electromagnon resonance in a helimagnet," Nature Communications, Nature, vol. 12(1), pages 1-7, December.
    8. Makiko Ogino & Yoshihiro Okamura & Kosuke Fujiwara & Takahiro Morimoto & Naoto Nagaosa & Yoshio Kaneko & Yoshinori Tokura & Youtarou Takahashi, 2024. "Terahertz photon to dc current conversion via magnetic excitations of multiferroics," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    9. Yakhno, V.G. & Yakhno, T.M., 2015. "Computing the fundamental solutions for equations of electrodynamics," Applied Mathematics and Computation, Elsevier, vol. 255(C), pages 189-195.

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