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Spin dynamics of the block orbital-selective Mott phase

Author

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  • J. Herbrych

    (University of Tennessee
    Oak Ridge National Laboratory)

  • N. Kaushal

    (University of Tennessee
    Oak Ridge National Laboratory)

  • A. Nocera

    (University of Tennessee
    Oak Ridge National Laboratory)

  • G. Alvarez

    (Oak Ridge National Laboratory
    Oak Ridge National Laboratory)

  • A. Moreo

    (University of Tennessee
    Oak Ridge National Laboratory)

  • E. Dagotto

    (University of Tennessee
    Oak Ridge National Laboratory)

Abstract

Iron-based superconductors display a variety of magnetic phases originating in the competition between electronic, orbital, and spin degrees of freedom. Previous theoretical investigations of the multi-orbital Hubbard model in one-dimension revealed the existence of an orbital-selective Mott phase (OSMP) with block spin order. Recent inelastic neutron scattering (INS) experiments on the BaFe2Se3 ladder compound confirmed the relevance of the block-OSMP. Moreover, the powder INS spectrum revealed an unexpected structure, containing both low-energy acoustic and high-energy optical modes. Here we present the theoretical prediction for the dynamical spin structure factor within a block-OSMP regime using the density-matrix renormalization-group method. In agreement with experiments, we find two dominant features: low-energy dispersive and high-energy dispersionless modes. We argue that the former represents the spin-wave-like dynamics of the block ferromagnetic islands, while the latter is attributed to a novel type of local on-site spin excitations controlled by the Hund coupling.

Suggested Citation

  • J. Herbrych & N. Kaushal & A. Nocera & G. Alvarez & A. Moreo & E. Dagotto, 2018. "Spin dynamics of the block orbital-selective Mott phase," Nature Communications, Nature, vol. 9(1), pages 1-10, December.
  • Handle: RePEc:nat:natcom:v:9:y:2018:i:1:d:10.1038_s41467-018-06181-6
    DOI: 10.1038/s41467-018-06181-6
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