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Experimental study of thermal rectification in suspended monolayer graphene

Author

Listed:
  • Haidong Wang

    (Kyushu University)

  • Shiqian Hu

    (Center for Phononics and Thermal Energy Science, School of Physics Science and Engineering, and Institute for Advanced Study, Tongji University
    China–EU Joint Lab for Nanophononics, School of Physics Science and Engineering, Tongji University
    Shanghai Key Laboratory of Special Artificial Microstructure Materials and Technology, School of Physics Science and Engineering, Tongji University)

  • Koji Takahashi

    (Kyushu University
    International Institute for Carbon-Neutral Energy Research (WPI-I2CNER), Kyushu University)

  • Xing Zhang

    (International Institute for Carbon-Neutral Energy Research (WPI-I2CNER), Kyushu University
    Tsinghua University)

  • Hiroshi Takamatsu

    (Kyushu University)

  • Jie Chen

    (Center for Phononics and Thermal Energy Science, School of Physics Science and Engineering, and Institute for Advanced Study, Tongji University
    China–EU Joint Lab for Nanophononics, School of Physics Science and Engineering, Tongji University
    Shanghai Key Laboratory of Special Artificial Microstructure Materials and Technology, School of Physics Science and Engineering, Tongji University)

Abstract

Thermal rectification is a fundamental phenomenon for active heat flow control. Significant thermal rectification is expected to exist in the asymmetric nanostructures, such as nanowires and thin films. As a one-atom-thick membrane, graphene has attracted much attention for realizing thermal rectification as shown by many molecular dynamics simulations. Here, we experimentally demonstrate thermal rectification in various asymmetric monolayer graphene nanostructures. A large thermal rectification factor of 26% is achieved in a defect-engineered monolayer graphene with nanopores on one side. A thermal rectification factor of 10% is achieved in a pristine monolayer graphene with nanoparticles deposited on one side or with a tapered width. The results indicate that the monolayer graphene has great potential to be used for designing high-performance thermal rectifiers for heat flow control and energy harvesting.

Suggested Citation

  • Haidong Wang & Shiqian Hu & Koji Takahashi & Xing Zhang & Hiroshi Takamatsu & Jie Chen, 2017. "Experimental study of thermal rectification in suspended monolayer graphene," Nature Communications, Nature, vol. 8(1), pages 1-8, August.
    • Handle: RePEc:nat:natcom:v:8:y:2017:i:1:d:10.1038_ncomms15843
    DOI: 10.1038/ncomms15843
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    Cited by:

    1. Klinar, K. & Kitanovski, A., 2020. "Thermal control elements for caloric energy conversion," Renewable and Sustainable Energy Reviews, Elsevier, vol. 118(C).
    2. Zhang, Ge & Cottrill, Anton L. & Koman, Volodymyr B. & Liu, Albert Tianxiang & Mahajan, Sayalee G. & Piephoff, D. Evan & Strano, Michael S., 2020. "Persistent, single-polarity energy harvesting from ambient thermal fluctuations using a thermal resonance device with thermal diodes," Applied Energy, Elsevier, vol. 280(C).
    3. Xiong, Kezhao & Zhou, Man & Liu, Wei & Zhang, Xiyun, 2024. "Regulating thermal rectification on random networks by depositing nanoparticles," Chaos, Solitons & Fractals, Elsevier, vol. 178(C).
    4. Mussad M. Alzahrani & Anurag Roy & Senthilarasu Sundaram & Tapas K. Mallick, 2021. "Investigation of Thermal Stress Arising in a Graphene Neutral Density Filter for Concentrated Photovoltaic System," Energies, MDPI, vol. 14(12), pages 1-9, June.

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