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Nonadditivity of critical Casimir forces

Author

Listed:
  • Sathyanarayana Paladugu

    (Soft Matter Lab, Bilkent University)

  • Agnese Callegari

    (Soft Matter Lab, Bilkent University)

  • Yazgan Tuna

    (Soft Matter Lab, Bilkent University
    UNAM—National Nanotechnology Research Center, Bilkent University)

  • Lukas Barth

    (Soft Matter Lab, Bilkent University)

  • Siegfried Dietrich

    (Max-Planck-Institut für Intelligente Systeme
    IV. Institut für Theoretische Physik, Universität Stuttgart)

  • Andrea Gambassi

    (SISSA—International School for Advanced Studies and INFN)

  • Giovanni Volpe

    (Soft Matter Lab, Bilkent University
    UNAM—National Nanotechnology Research Center, Bilkent University)

Abstract

In soft condensed matter physics, effective interactions often emerge due to the spatial confinement of fluctuating fields. For instance, microscopic particles dissolved in a binary liquid mixture are subject to critical Casimir forces whenever their surfaces confine the thermal fluctuations of the order parameter of the solvent close to its critical demixing point. These forces are theoretically predicted to be nonadditive on the scale set by the bulk correlation length of the fluctuations. Here we provide direct experimental evidence of this fact by reporting the measurement of the associated many-body forces. We consider three colloidal particles in optical traps and observe that the critical Casimir force exerted on one of them by the other two differs from the sum of the forces they exert separately. This three-body effect depends sensitively on the distance from the critical point and on the chemical functionalisation of the colloid surfaces.

Suggested Citation

  • Sathyanarayana Paladugu & Agnese Callegari & Yazgan Tuna & Lukas Barth & Siegfried Dietrich & Andrea Gambassi & Giovanni Volpe, 2016. "Nonadditivity of critical Casimir forces," Nature Communications, Nature, vol. 7(1), pages 1-8, September.
    • Handle: RePEc:nat:natcom:v:7:y:2016:i:1:d:10.1038_ncomms11403
    DOI: 10.1038/ncomms11403
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    Cited by:

    1. Jens Grauer & Falko Schmidt & Jesús Pineda & Benjamin Midtvedt & Hartmut Löwen & Giovanni Volpe & Benno Liebchen, 2021. "Active droploids," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    2. Gnan, Nicoletta, 2023. "Lecture notes of the 15th international summer school on Fundamental Problems in Statistical Physics: Colloidal dispersions," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 631(C).
    3. Gan Wang & Piotr Nowakowski & Nima Farahmand Bafi & Benjamin Midtvedt & Falko Schmidt & Agnese Callegari & Ruggero Verre & Mikael Käll & S. Dietrich & Svyatoslav Kondrat & Giovanni Volpe, 2024. "Nanoalignment by critical Casimir torques," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    4. Dantchev, Daniel & Vassilev, Vassil M. & Djondjorov, Peter A., 2018. "Analytical results for the Casimir force in a Ginzburg–Landau type model of a film with strongly adsorbing competing walls," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 510(C), pages 302-315.

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