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Macrospin dynamics in antiferromagnets triggered by sub-20 femtosecond injection of nanomagnons

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  • D. Bossini

    (Institute for Molecules and Materials, Spectroscopy of Solids and Interfaces, Radboud University
    Present address: Institute for Photon Science and Technology Graduate School of Science, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033, Japan)

  • S. Dal Conte

    (Politecnico di Milano
    Istituto di Fotonica e Nanotecnologie, Consiglio Nazionale delle Ricerche)

  • Y. Hashimoto

    (Institute for Molecules and Materials, Spectroscopy of Solids and Interfaces, Radboud University
    Present address: Spin Quantum Rectification Project, ERATO, Japan Science and Technology Agency, Sendai 980-8577, Japan)

  • A. Secchi

    (Institute for Molecules and Materials, Spectroscopy of Solids and Interfaces, Radboud University)

  • R. V. Pisarev

    (Ioffe Physical-Technical Institute, Ferroics Physics Laboratory, Russian Academy of Sciences)

  • Th. Rasing

    (Institute for Molecules and Materials, Spectroscopy of Solids and Interfaces, Radboud University)

  • G. Cerullo

    (Politecnico di Milano
    Istituto di Fotonica e Nanotecnologie, Consiglio Nazionale delle Ricerche)

  • A. V. Kimel

    (Institute for Molecules and Materials, Spectroscopy of Solids and Interfaces, Radboud University)

Abstract

The understanding of how the sub-nanoscale exchange interaction evolves in macroscale correlations and ordered phases of matter, such as magnetism and superconductivity, requires to bridging the quantum and classical worlds. This monumental challenge has so far only been achieved for systems close to their thermodynamical equilibrium. Here we follow in real time the ultrafast dynamics of the macroscale magnetic order parameter in the Heisenberg antiferromagnet KNiF3 triggered by the impulsive optical generation of spin excitations with the shortest possible nanometre wavelength and femtosecond period. Our magneto-optical pump–probe experiments also demonstrate the coherent manipulation of the phase and amplitude of these femtosecond nanomagnons, whose frequencies are defined by the exchange energy. These findings open up opportunities for fundamental research on the role of short-wavelength spin excitations in magnetism and strongly correlated materials; they also suggest that nanospintronics and nanomagnonics can employ coherently controllable spin waves with frequencies in the 20 THz domain.

Suggested Citation

  • D. Bossini & S. Dal Conte & Y. Hashimoto & A. Secchi & R. V. Pisarev & Th. Rasing & G. Cerullo & A. V. Kimel, 2016. "Macrospin dynamics in antiferromagnets triggered by sub-20 femtosecond injection of nanomagnons," Nature Communications, Nature, vol. 7(1), pages 1-8, April.
  • Handle: RePEc:nat:natcom:v:7:y:2016:i:1:d:10.1038_ncomms10645
    DOI: 10.1038/ncomms10645
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    Cited by:

    1. Farhan Nur Kholid & Dominik Hamara & Ahmad Faisal Bin Hamdan & Guillermo Nava Antonio & Richard Bowen & Dorothée Petit & Russell Cowburn & Roman V. Pisarev & Davide Bossini & Joseph Barker & Chiara Ci, 2023. "The importance of the interface for picosecond spin pumping in antiferromagnet-heavy metal heterostructures," Nature Communications, Nature, vol. 14(1), pages 1-8, December.

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