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Spectral splitting photovoltaics using perovskite and wideband dye-sensitized solar cells

Author

Listed:
  • Takumi Kinoshita

    (Research Center for Advanced Science and Technology (RCAST), The University of Tokyo)

  • Kazuteru Nonomura

    (Laboratory of Photomolecular Science, Swiss Federal Institute of Technology)

  • Nam Joong Jeon

    (Korea Research Institute of Chemical Technology)

  • Fabrizio Giordano

    (Laboratory of Photonics and Interfaces, Swiss Federal Institute of Technology)

  • Antonio Abate

    (Laboratory of Photonics and Interfaces, Swiss Federal Institute of Technology)

  • Satoshi Uchida

    (Komaba Organization for Educational Excellence (KOMEX), The University of Tokyo)

  • Takaya Kubo

    (Research Center for Advanced Science and Technology (RCAST), The University of Tokyo)

  • Sang Il Seok

    (Korea Research Institute of Chemical Technology
    School of Energy and Chemical Engineering, Ulsan National Institute of Science and Technology (UNIST), 50 UNIST-gil, Eonyang-eup, Ulju-gun, Ulsan 689-798, Korea)

  • Mohammad Khaja Nazeeruddin

    (Laboratory of Photonics and Interfaces, Swiss Federal Institute of Technology)

  • Anders Hagfeldt

    (Laboratory of Photomolecular Science, Swiss Federal Institute of Technology)

  • Michael Grätzel

    (Laboratory of Photonics and Interfaces, Swiss Federal Institute of Technology)

  • Hiroshi Segawa

    (Research Center for Advanced Science and Technology (RCAST), The University of Tokyo)

Abstract

The extension of the light absorption of photovoltaics into the near-infrared region is important to increase the energy conversion efficiency. Although the progress of the lead halide perovskite solar cells is remarkable, and high conversion efficiency of >20% has been reached, their absorption limit on the long-wavelength side is ∼800 nm. To further enhance the conversion efficiency of perovskite-based photovoltaics, a hybridized system with near-infrared photovoltaics is a useful approach. Here we report a panchromatic sensitizer, coded DX3, that exhibits a broad response into the near-infrared, up to ∼1100 nm, and a photocurrent density exceeding 30 mA cm−2 in simulated air mass 1.5 standard solar radiation. Using the DX3-based dye-sensitized solar cell in conjunction with a perovskite cell that harvests visible light, the hybridized mesoscopic photovoltaics achieved a conversion efficiency of 21.5% using a system of spectral splitting.

Suggested Citation

  • Takumi Kinoshita & Kazuteru Nonomura & Nam Joong Jeon & Fabrizio Giordano & Antonio Abate & Satoshi Uchida & Takaya Kubo & Sang Il Seok & Mohammad Khaja Nazeeruddin & Anders Hagfeldt & Michael Grätzel, 2015. "Spectral splitting photovoltaics using perovskite and wideband dye-sensitized solar cells," Nature Communications, Nature, vol. 6(1), pages 1-8, December.
    • Handle: RePEc:nat:natcom:v:6:y:2015:i:1:d:10.1038_ncomms9834
    DOI: 10.1038/ncomms9834
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    Cited by:

    1. Wali, Qamar & Elumalai, Naveen Kumar & Iqbal, Yaseen & Uddin, Ashraf & Jose, Rajan, 2018. "Tandem perovskite solar cells," Renewable and Sustainable Energy Reviews, Elsevier, vol. 84(C), pages 89-110.
    2. Matthias Kick & Ezra Alexander & Anton Beiersdorfer & Troy Voorhis, 2024. "Super-resolution techniques to simulate electronic spectra of large molecular systems," Nature Communications, Nature, vol. 15(1), pages 1-11, December.

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