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Tuning the band structure and superconductivity in single-layer FeSe by interface engineering

Author

Listed:
  • R. Peng

    (State Key Laboratory of Surface Physics, Fudan University
    Advanced Materials Laboratory, Fudan University)

  • H. C. Xu

    (State Key Laboratory of Surface Physics, Fudan University
    Advanced Materials Laboratory, Fudan University)

  • S. Y. Tan

    (State Key Laboratory of Surface Physics, Fudan University
    Advanced Materials Laboratory, Fudan University)

  • H. Y. Cao

    (State Key Laboratory of Surface Physics, Fudan University
    Key Laboratory for Computational Physical Sciences (Ministry of Education), Fudan University)

  • M. Xia

    (State Key Laboratory of Surface Physics, Fudan University
    Advanced Materials Laboratory, Fudan University)

  • X. P. Shen

    (State Key Laboratory of Surface Physics, Fudan University
    Advanced Materials Laboratory, Fudan University)

  • Z. C. Huang

    (State Key Laboratory of Surface Physics, Fudan University
    Advanced Materials Laboratory, Fudan University)

  • C.H.P. Wen

    (State Key Laboratory of Surface Physics, Fudan University
    Advanced Materials Laboratory, Fudan University)

  • Q. Song

    (State Key Laboratory of Surface Physics, Fudan University
    Advanced Materials Laboratory, Fudan University)

  • T. Zhang

    (State Key Laboratory of Surface Physics, Fudan University
    Advanced Materials Laboratory, Fudan University)

  • B. P. Xie

    (State Key Laboratory of Surface Physics, Fudan University
    Advanced Materials Laboratory, Fudan University)

  • X. G. Gong

    (State Key Laboratory of Surface Physics, Fudan University
    Key Laboratory for Computational Physical Sciences (Ministry of Education), Fudan University)

  • D. L. Feng

    (State Key Laboratory of Surface Physics, Fudan University
    Advanced Materials Laboratory, Fudan University)

Abstract

The interface between transition metal compounds provides a rich playground for emergent phenomena. Recently, significantly enhanced superconductivity has been reported for single-layer FeSe on Nb-doped SrTiO3 substrate. Yet it remains mysterious how the interface affects the superconductivity. Here we use in situ angle-resolved photoemission spectroscopy to investigate various FeSe-based heterostructures grown by molecular beam epitaxy, and uncover that electronic correlations and superconducting gap-closing temperature (Tg) are tuned by interfacial effects. Tg up to 75 K is observed in extremely tensile-strained single-layer FeSe on Nb-doped BaTiO3, which sets a record high pairing temperature for both Fe-based superconductor and monolayer-thick films, providing a promising prospect on realizing more cost-effective superconducting device. Moreover, our results exclude the direct correlation between superconductivity and tensile strain or the energy of an interfacial phonon mode, and highlight the critical and non-trivial role of FeSe/oxide interface on the high Tg, which provides new clues for understanding its origin.

Suggested Citation

  • R. Peng & H. C. Xu & S. Y. Tan & H. Y. Cao & M. Xia & X. P. Shen & Z. C. Huang & C.H.P. Wen & Q. Song & T. Zhang & B. P. Xie & X. G. Gong & D. L. Feng, 2014. "Tuning the band structure and superconductivity in single-layer FeSe by interface engineering," Nature Communications, Nature, vol. 5(1), pages 1-7, December.
  • Handle: RePEc:nat:natcom:v:5:y:2014:i:1:d:10.1038_ncomms6044
    DOI: 10.1038/ncomms6044
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    Cited by:

    1. Yuanhe Song & Zheng Chen & Qinghua Zhang & Haichao Xu & Xia Lou & Xiaoyang Chen & Xiaofeng Xu & Xuetao Zhu & Ran Tao & Tianlun Yu & Hao Ru & Yihua Wang & Tong Zhang & Jiandong Guo & Lin Gu & Yanwu Xie, 2021. "High temperature superconductivity at FeSe/LaFeO3 interface," Nature Communications, Nature, vol. 12(1), pages 1-8, December.

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