Author
Listed:
- R. Peng
(State Key Laboratory of Surface Physics, Fudan University
Advanced Materials Laboratory, Fudan University)
- H. C. Xu
(State Key Laboratory of Surface Physics, Fudan University
Advanced Materials Laboratory, Fudan University)
- S. Y. Tan
(State Key Laboratory of Surface Physics, Fudan University
Advanced Materials Laboratory, Fudan University)
- H. Y. Cao
(State Key Laboratory of Surface Physics, Fudan University
Key Laboratory for Computational Physical Sciences (Ministry of Education), Fudan University)
- M. Xia
(State Key Laboratory of Surface Physics, Fudan University
Advanced Materials Laboratory, Fudan University)
- X. P. Shen
(State Key Laboratory of Surface Physics, Fudan University
Advanced Materials Laboratory, Fudan University)
- Z. C. Huang
(State Key Laboratory of Surface Physics, Fudan University
Advanced Materials Laboratory, Fudan University)
- C.H.P. Wen
(State Key Laboratory of Surface Physics, Fudan University
Advanced Materials Laboratory, Fudan University)
- Q. Song
(State Key Laboratory of Surface Physics, Fudan University
Advanced Materials Laboratory, Fudan University)
- T. Zhang
(State Key Laboratory of Surface Physics, Fudan University
Advanced Materials Laboratory, Fudan University)
- B. P. Xie
(State Key Laboratory of Surface Physics, Fudan University
Advanced Materials Laboratory, Fudan University)
- X. G. Gong
(State Key Laboratory of Surface Physics, Fudan University
Key Laboratory for Computational Physical Sciences (Ministry of Education), Fudan University)
- D. L. Feng
(State Key Laboratory of Surface Physics, Fudan University
Advanced Materials Laboratory, Fudan University)
Abstract
The interface between transition metal compounds provides a rich playground for emergent phenomena. Recently, significantly enhanced superconductivity has been reported for single-layer FeSe on Nb-doped SrTiO3 substrate. Yet it remains mysterious how the interface affects the superconductivity. Here we use in situ angle-resolved photoemission spectroscopy to investigate various FeSe-based heterostructures grown by molecular beam epitaxy, and uncover that electronic correlations and superconducting gap-closing temperature (Tg) are tuned by interfacial effects. Tg up to 75 K is observed in extremely tensile-strained single-layer FeSe on Nb-doped BaTiO3, which sets a record high pairing temperature for both Fe-based superconductor and monolayer-thick films, providing a promising prospect on realizing more cost-effective superconducting device. Moreover, our results exclude the direct correlation between superconductivity and tensile strain or the energy of an interfacial phonon mode, and highlight the critical and non-trivial role of FeSe/oxide interface on the high Tg, which provides new clues for understanding its origin.
Suggested Citation
R. Peng & H. C. Xu & S. Y. Tan & H. Y. Cao & M. Xia & X. P. Shen & Z. C. Huang & C.H.P. Wen & Q. Song & T. Zhang & B. P. Xie & X. G. Gong & D. L. Feng, 2014.
"Tuning the band structure and superconductivity in single-layer FeSe by interface engineering,"
Nature Communications, Nature, vol. 5(1), pages 1-7, December.
Handle:
RePEc:nat:natcom:v:5:y:2014:i:1:d:10.1038_ncomms6044
DOI: 10.1038/ncomms6044
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