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A room temperature low-threshold ultraviolet plasmonic nanolaser

Author

Listed:
  • Qing Zhang

    (School of Physical and Mathematical Sciences, Nanyang Technological University)

  • Guangyuan Li

    (School of Physical and Mathematical Sciences, Nanyang Technological University)

  • Xinfeng Liu

    (School of Physical and Mathematical Sciences, Nanyang Technological University)

  • Fang Qian

    (Physical and Life Sciences Directorate, Lawrence Livermore National Laboratory)

  • Yat Li

    (University of California)

  • Tze Chien Sum

    (School of Physical and Mathematical Sciences, Nanyang Technological University
    Singapore-Berkeley Research Initiative for Sustainable Energy)

  • Charles M. Lieber

    (Harvard University)

  • Qihua Xiong

    (School of Physical and Mathematical Sciences, Nanyang Technological University
    NOVITAS, Nanoelectronics Centre of Excellence, School of Electrical and Electronic Engineering, Nanyang Technological University)

Abstract

Constrained by large ohmic and radiation losses, plasmonic nanolasers operated at visible regime are usually achieved either with a high threshold (102–104 MW cm−2) or at cryogenic temperatures (4–120 K). Particularly, the bending-back effect of surface plasmon (SP) dispersion at high energy makes the SP lasing below 450 nm more challenging. Here we demonstrate the first strong room temperature ultraviolet (~370 nm) SP polariton laser with an extremely low threshold (~3.5 MW cm−2). We find that a closed-contact planar semiconductor–insulator–metal interface greatly lessens the scattering loss, and more importantly, efficiently promotes the exciton–SP energy transfer thus furnishes adequate optical gain to compensate the loss. An excitation polarization-dependent lasing action is observed and interpreted with a microscopic energy-transfer process from excitons to SPs. Our work advances the fundamental understanding of hybrid plasmonic waveguide laser and provides a solution of realizing room temperature UV nanolasers for biological applications and information technologies.

Suggested Citation

  • Qing Zhang & Guangyuan Li & Xinfeng Liu & Fang Qian & Yat Li & Tze Chien Sum & Charles M. Lieber & Qihua Xiong, 2014. "A room temperature low-threshold ultraviolet plasmonic nanolaser," Nature Communications, Nature, vol. 5(1), pages 1-9, December.
  • Handle: RePEc:nat:natcom:v:5:y:2014:i:1:d:10.1038_ncomms5953
    DOI: 10.1038/ncomms5953
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    Cited by:

    1. Yang-Chun Lee & Ya-Lun Ho & Bo-Wei Lin & Mu-Hsin Chen & Di Xing & Hirofumi Daiguji & Jean-Jacques Delaunay, 2023. "High-Q lasing via all-dielectric Bloch-surface-wave platform," Nature Communications, Nature, vol. 14(1), pages 1-10, December.

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