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Unusual ultra-low-frequency fluctuations in freestanding graphene

Author

Listed:
  • P. Xu

    (University of Arkansas)

  • M. Neek-Amal

    (Departement Fysica, Universiteit Antwerpen
    Shahid Rajaee Teacher Training University)

  • S. D. Barber

    (University of Arkansas)

  • J. K. Schoelz

    (University of Arkansas)

  • M. L. Ackerman

    (University of Arkansas)

  • P. M. Thibado

    (University of Arkansas)

  • A. Sadeghi

    (Departement Physik, Universat Basel)

  • F. M. Peeters

    (Departement Fysica, Universiteit Antwerpen)

Abstract

Intrinsic ripples in freestanding graphene have been exceedingly difficult to study. Individual ripple geometry was recently imaged using scanning tunnelling microscopy, but these measurements are limited to static configurations. Thermally-activated flexural phonon modes should generate dynamic changes in curvature. Here we show how to track the vertical movement of a one-square-angstrom region of freestanding graphene using scanning tunnelling microscopy, thereby allowing measurement of the out-of-plane time trajectory and fluctuations over long time periods. We also present a model from elasticity theory to explain the very-low-frequency oscillations. Unexpectedly, we sometimes detect a sudden colossal jump, which we interpret as due to mirror buckling. This innovative technique provides a much needed atomic-scale probe for the time-dependent behaviours of intrinsic ripples. The discovery of this novel progenitor represents a fundamental advance in the use of scanning tunnelling microscopy, which together with the application of a thermal load provides a low-frequency nano-resonator.

Suggested Citation

  • P. Xu & M. Neek-Amal & S. D. Barber & J. K. Schoelz & M. L. Ackerman & P. M. Thibado & A. Sadeghi & F. M. Peeters, 2014. "Unusual ultra-low-frequency fluctuations in freestanding graphene," Nature Communications, Nature, vol. 5(1), pages 1-7, September.
  • Handle: RePEc:nat:natcom:v:5:y:2014:i:1:d:10.1038_ncomms4720
    DOI: 10.1038/ncomms4720
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    Cited by:

    1. Yue Kai & Wenlong Xu & Bailin Zheng & Nan Yang & Kai Zhang & P. M. Thibado, 2019. "Origin of Non-Gaussian Velocity Distribution Found in Freestanding Graphene Membranes," Complexity, Hindawi, vol. 2019, pages 1-7, March.

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