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Observation of a large spin-dependent transport length in organic spin valves at room temperature

Author

Listed:
  • Xianmin Zhang

    (World Premier International Research Center, Advanced Institute for Materials Research, Tohoku University)

  • Shigemi Mizukami

    (World Premier International Research Center, Advanced Institute for Materials Research, Tohoku University)

  • Takahide Kubota

    (World Premier International Research Center, Advanced Institute for Materials Research, Tohoku University)

  • Qinli Ma

    (World Premier International Research Center, Advanced Institute for Materials Research, Tohoku University)

  • Mikihiko Oogane

    (Tohoku University)

  • Hiroshi Naganuma

    (Tohoku University)

  • Yasuo Ando

    (Tohoku University)

  • Terunobu Miyazaki

    (World Premier International Research Center, Advanced Institute for Materials Research, Tohoku University)

Abstract

The integration of organic semiconductors and magnetism has been a fascinating topic for fundamental scientific research and future applications in electronics, because organic semiconductors are expected to possess a large spin-dependent transport length based on weak spin–orbit coupling and weak hyperfine interaction. However, to date, this length has typically been limited to several nanometres at room temperature, and a large length has only been observed at low temperatures. Here we report on a novel organic spin valve device using C60 as the spacer layer. A magnetoresistance ratio of over 5% was observed at room temperature, which is one of the highest magnetoresistance ratios ever reported. Most importantly, a large spin-dependent transport length of approximately 110 nm was experimentally observed for the C60 layer at room temperature. These results provide insights for further understanding spin transport in organic semiconductors and may strongly advance the development of spin-based organic devices.

Suggested Citation

  • Xianmin Zhang & Shigemi Mizukami & Takahide Kubota & Qinli Ma & Mikihiko Oogane & Hiroshi Naganuma & Yasuo Ando & Terunobu Miyazaki, 2013. "Observation of a large spin-dependent transport length in organic spin valves at room temperature," Nature Communications, Nature, vol. 4(1), pages 1-7, June.
  • Handle: RePEc:nat:natcom:v:4:y:2013:i:1:d:10.1038_ncomms2423
    DOI: 10.1038/ncomms2423
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    Cited by:

    1. Xueli Yang & Ankang Guo & Jie Yang & Jinyang Chen & Ke Meng & Shunhua Hu & Ran Duan & Mingliang Zhu & Wenkang Shi & Yang Qin & Rui Zhang & Haijun Yang & Jikun Li & Lidan Guo & Xiangnan Sun & Yunqi Liu, 2024. "Halogenated-edge polymeric semiconductor for efficient spin transport," Nature Communications, Nature, vol. 15(1), pages 1-11, December.

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