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Space-based observations of tropospheric ethane map emissions from fossil fuel extraction

Author

Listed:
  • Jared F. Brewer

    (and Climate)

  • Dylan B. Millet

    (and Climate)

  • Kelley C. Wells

    (and Climate)

  • Vivienne H. Payne

    (California Institute of Technology)

  • Susan Kulawik

    (BAER Institute)

  • Corinne Vigouroux

    (Royal Belgian Institute for Space Aeronomy (BIRA-IASB))

  • Karen E. Cady-Pereira

    (Atmospheric and Environmental Research)

  • Rick Pernak

    (Atmospheric and Environmental Research)

  • Minqiang Zhou

    (Chinese Academy of Sciences)

Abstract

Ethane is the most abundant non-methane hydrocarbon in the troposphere, where it impacts ozone and reactive nitrogen and is a key tracer used for partitioning emitted methane between anthropogenic and natural sources. However, quantification has been challenged by sparse observations. Here, we present a satellite-based measurement of tropospheric ethane and demonstrate its utility for fossil-fuel source quantification. An ethane spectral signal is detectable from space in Cross-track Infrared Sounder (CrIS) radiances, revealing ethane signatures associated with fires and fossil fuel production. We use machine-learning to convert these signals to ethane abundances and validate the results against surface observations (R2 = 0.66, mean CrIS/surface ratio: 0.65). The CrIS data show that the Permian Basin in Texas and New Mexico exhibits the largest persistent ethane enhancements on the planet, with regional emissions underestimated by seven-fold. Correcting this underestimate reveals Permian ethane emissions that represent at least 4-7% of the global fossil-fuel ethane source.

Suggested Citation

  • Jared F. Brewer & Dylan B. Millet & Kelley C. Wells & Vivienne H. Payne & Susan Kulawik & Corinne Vigouroux & Karen E. Cady-Pereira & Rick Pernak & Minqiang Zhou, 2024. "Space-based observations of tropospheric ethane map emissions from fossil fuel extraction," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
  • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-52247-z
    DOI: 10.1038/s41467-024-52247-z
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    References listed on IDEAS

    as
    1. Federico Maddanu & Tommaso Proietti, 2023. "Trends in atmospheric ethane," Climatic Change, Springer, vol. 176(5), pages 1-23, May.
    2. Isobel J. Simpson & Mads P. Sulbaek Andersen & Simone Meinardi & Lori Bruhwiler & Nicola J. Blake & Detlev Helmig & F. Sherwood Rowland & Donald R. Blake, 2012. "Long-term decline of global atmospheric ethane concentrations and implications for methane," Nature, Nature, vol. 488(7412), pages 490-494, August.
    3. Kelley C. Wells & Dylan B. Millet & Vivienne H. Payne & M. Julian Deventer & Kelvin H. Bates & Joost A. Gouw & Martin Graus & Carsten Warneke & Armin Wisthaler & Jose D. Fuentes, 2020. "Satellite isoprene retrievals constrain emissions and atmospheric oxidation," Nature, Nature, vol. 585(7824), pages 225-233, September.
    4. Bruno Franco & Lieven Clarisse & Martin Van Damme & Juliette Hadji-Lazaro & Cathy Clerbaux & Pierre-François Coheur, 2022. "Ethylene industrial emitters seen from space," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
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