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Switchable unidirectional emissions from hydrogel gratings with integrated carbon quantum dots

Author

Listed:
  • Chenjie Dai

    (Wuhan University)

  • Shuai Wan

    (Wuhan University)

  • Zhe Li

    (Wuhan University)

  • Yangyang Shi

    (Wuhan University)

  • Shuang Zhang

    (The University of Hong Kong)

  • Zhongyang Li

    (Wuhan University
    Wuhan Institute of Quantum Technology
    Wuhan University
    Suzhou Institute of Wuhan University)

Abstract

Directional emission of photoluminescence despite its incoherence is an attractive technique for light-emitting fields and nanophotonics. Optical metasurfaces provide a promising route for wavefront engineering at the subwavelength scale, enabling the feasibility of unidirectional emission. However, current directional emission strategies are mostly based on static metasurfaces, and it remains a challenge to achieve unidirectional emissions tuning with high performance. Here, we demonstrate quantum dots-hydrogel integrated gratings for actively switchable unidirectional emission with simultaneously a narrow divergence angle less than 1.5° and a large diffraction angle greater than 45°. We further demonstrate that the grating efficiency alteration leads to a more than 7-fold tuning of emission intensity at diffraction order due to the variation of hydrogel morphology subject to change in ambient humidity. Our proposed switchable emission strategy can promote technologies of active light-emitting devices for radiation control and optical imaging.

Suggested Citation

  • Chenjie Dai & Shuai Wan & Zhe Li & Yangyang Shi & Shuang Zhang & Zhongyang Li, 2024. "Switchable unidirectional emissions from hydrogel gratings with integrated carbon quantum dots," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
  • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-45284-1
    DOI: 10.1038/s41467-024-45284-1
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    References listed on IDEAS

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    1. Yahya Mohtashami & Ryan A. DeCrescent & Larry K. Heki & Prasad P. Iyer & Nikita A. Butakov & Matthew S. Wong & Abdullah Alhassan & William J. Mitchell & Shuji Nakamura & Steven P. DenBaars & Jon. A. S, 2021. "Light-emitting metalenses and meta-axicons for focusing and beaming of spontaneous emission," Nature Communications, Nature, vol. 12(1), pages 1-7, December.
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    Cited by:

    1. Jongsun Yoon & Chunghwan Jung & Jaekyung Kim & Junsuk Rho & Hyomin Lee, 2024. "Chemically and geometrically programmable photoreactive polymers for transformational humidity-sensitive full-color devices," Nature Communications, Nature, vol. 15(1), pages 1-11, December.

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