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Modulation of perovskite degradation with multiple-barrier for light-heat stable perovskite solar cells

Author

Listed:
  • Jing Zhou

    (Huazhong University of Science and Technology (HUST))

  • Zonghao Liu

    (Huazhong University of Science and Technology (HUST)
    Optics Valley Laboratory)

  • Peng Yu

    (Huazhong University of Science and Technology (HUST)
    Huazhong University of Science and Technology)

  • Guoqing Tong

    (Okinawa Institutes of Science and Technology Graduate University (OIST))

  • Ruijun Chen

    (Huanggang Normal University)

  • Luis K. Ono

    (Okinawa Institutes of Science and Technology Graduate University (OIST))

  • Rui Chen

    (Huazhong University of Science and Technology (HUST))

  • Haixin Wang

    (Huazhong University of Science and Technology (HUST))

  • Fumeng Ren

    (Huazhong University of Science and Technology (HUST))

  • Sanwan Liu

    (Huazhong University of Science and Technology (HUST))

  • Jianan Wang

    (Huazhong University of Science and Technology (HUST))

  • Zhigao Lan

    (Huanggang Normal University)

  • Yabing Qi

    (Okinawa Institutes of Science and Technology Graduate University (OIST))

  • Wei Chen

    (Huazhong University of Science and Technology (HUST)
    Optics Valley Laboratory)

Abstract

The long-term stability of perovskite solar cells remains one of the most important challenges for the commercialization of this emerging photovoltaic technology. Here, we adopt a non-noble metal/metal oxide/polymer multiple-barrier to suppress the halide consumption and gaseous perovskite decomposition products release with the chemically inert bismuth electrode and Al2O3/parylene thin-film encapsulation, as well as the tightly closed system created by the multiple-barrier to jointly suppress the degradation of perovskite solar cells, allowing the corresponding decomposition reactions to reach benign equilibria. The resulting encapsulated formamidinium cesium-based perovskite solar cells with multiple-barrier maintain 90% of their initial efficiencies after continuous operation at 45 °C for 5200 h and 93% of their initial efficiency after continuous operation at 75 °C for 1000 h under 1 sun equivalent white-light LED illumination.

Suggested Citation

  • Jing Zhou & Zonghao Liu & Peng Yu & Guoqing Tong & Ruijun Chen & Luis K. Ono & Rui Chen & Haixin Wang & Fumeng Ren & Sanwan Liu & Jianan Wang & Zhigao Lan & Yabing Qi & Wei Chen, 2023. "Modulation of perovskite degradation with multiple-barrier for light-heat stable perovskite solar cells," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-41856-9
    DOI: 10.1038/s41467-023-41856-9
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    Cited by:

    1. Shuxian Du & Hao Huang & Zhineng Lan & Peng Cui & Liang Li & Min Wang & Shujie Qu & Luyao Yan & Changxu Sun & Yingying Yang & Xinxin Wang & Meicheng Li, 2024. "Inhibiting perovskite decomposition by a creeper-inspired strategy enables efficient and stable perovskite solar cells," Nature Communications, Nature, vol. 15(1), pages 1-11, December.

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