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Anisotropy-driven quantum criticality in an intermediate valence system

Author

Listed:
  • Mihael S. Grbić

    (University of Tokyo
    University of Zagreb)

  • Eoin C. T. O’Farrell

    (University of Tokyo)

  • Yosuke Matsumoto

    (University of Tokyo)

  • Kentaro Kuga

    (University of Tokyo)

  • Manuel Brando

    (Max Planck Institute for Chemical Physics of Solids)

  • Robert Küchler

    (Max Planck Institute for Chemical Physics of Solids)

  • Andriy H. Nevidomskyy

    (Rice University)

  • Makoto Yoshida

    (University of Tokyo)

  • Toshiro Sakakibara

    (University of Tokyo)

  • Yohei Kono

    (University of Tokyo)

  • Yasuyuki Shimura

    (University of Tokyo)

  • Michael L. Sutherland

    (University of Cambridge)

  • Masashi Takigawa

    (University of Tokyo)

  • Satoru Nakatsuji

    (University of Tokyo
    The University of Tokyo
    CREST, Japan Science and Technology Agency (JST)
    Johns Hopkins University)

Abstract

Intermetallic compounds containing f-electron elements have been prototypical materials for investigating strong electron correlations and quantum criticality (QC). Their heavy fermion ground state evoked by the magnetic f-electrons is susceptible to the onset of quantum phases, such as magnetism or superconductivity, due to the enhanced effective mass (m*) and a corresponding decrease of the Fermi temperature. However, the presence of f-electron valence fluctuations to a non-magnetic state is regarded an anathema to QC, as it usually generates a paramagnetic Fermi-liquid state with quasiparticles of moderate m*. Such systems are typically isotropic, with a characteristic energy scale T0 of the order of hundreds of kelvins that require large magnetic fields or pressures to promote a valence or magnetic instability. Here we show the discovery of a quantum critical behaviour and a Lifshitz transition under low magnetic field in an intermediate valence compound α-YbAlB4. The QC origin is attributed to the anisotropic hybridization between the conduction and localized f-electrons. These findings suggest a new route to bypass the large valence energy scale in developing the QC.

Suggested Citation

  • Mihael S. Grbić & Eoin C. T. O’Farrell & Yosuke Matsumoto & Kentaro Kuga & Manuel Brando & Robert Küchler & Andriy H. Nevidomskyy & Makoto Yoshida & Toshiro Sakakibara & Yohei Kono & Yasuyuki Shimura , 2022. "Anisotropy-driven quantum criticality in an intermediate valence system," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-29757-9
    DOI: 10.1038/s41467-022-29757-9
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    References listed on IDEAS

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    1. J. Custers & P. Gegenwart & H. Wilhelm & K. Neumaier & Y. Tokiwa & O. Trovarelli & C. Geibel & F. Steglich & C. Pépin & P. Coleman, 2003. "The break-up of heavy electrons at a quantum critical point," Nature, Nature, vol. 424(6948), pages 524-527, July.
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