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Motional narrowing, ballistic transport, and trapping of room-temperature exciton polaritons in an atomically-thin semiconductor

Author

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  • M. Wurdack

    (The Australian National University)

  • E. Estrecho

    (The Australian National University)

  • S. Todd

    (The Australian National University)

  • T. Yun

    (The Australian National University)

  • M. Pieczarka

    (The Australian National University
    Wrocław University of Science and Technology)

  • S. K. Earl

    (Swinburne University of Technology)

  • J. A. Davis

    (Swinburne University of Technology)

  • C. Schneider

    (Carl von Ossietzky Universität Oldenburg)

  • A. G. Truscott

    (The Australian National University)

  • E. A. Ostrovskaya

    (The Australian National University)

Abstract

Monolayer transition metal dichalcogenide crystals (TMDCs) hold great promise for semiconductor optoelectronics because their bound electron-hole pairs (excitons) are stable at room temperature and interact strongly with light. When TMDCs are embedded in an optical microcavity, excitons can hybridise with cavity photons to form exciton polaritons, which inherit useful properties from their constituents. The ability to manipulate and trap polaritons on a microchip is critical for applications. Here, we create a non-trivial potential landscape for polaritons in monolayer WS2, and demonstrate their trapping and ballistic propagation across tens of micrometers. We show that the effects of dielectric disorder, which restrict the diffusion of WS2 excitons and broaden their spectral resonance, are dramatically reduced for polaritons, leading to motional narrowing and preserved partial coherence. Linewidth narrowing and coherence are further enhanced in the trap. Our results demonstrate the possibility of long-range dissipationless transport and efficient trapping of TMDC polaritons in ambient conditions.

Suggested Citation

  • M. Wurdack & E. Estrecho & S. Todd & T. Yun & M. Pieczarka & S. K. Earl & J. A. Davis & C. Schneider & A. G. Truscott & E. A. Ostrovskaya, 2021. "Motional narrowing, ballistic transport, and trapping of room-temperature exciton polaritons in an atomically-thin semiconductor," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:12:y:2021:i:1:d:10.1038_s41467-021-25656-7
    DOI: 10.1038/s41467-021-25656-7
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    Cited by:

    1. Jiaxin Zhao & Antonio Fieramosca & Kevin Dini & Ruiqi Bao & Wei Du & Rui Su & Yuan Luo & Weijie Zhao & Daniele Sanvitto & Timothy C. H. Liew & Qihua Xiong, 2023. "Exciton polariton interactions in Van der Waals superlattices at room temperature," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    2. M. Wurdack & T. Yun & M. Katzer & A. G. Truscott & A. Knorr & M. Selig & E. A. Ostrovskaya & E. Estrecho, 2023. "Negative-mass exciton polaritons induced by dissipative light-matter coupling in an atomically thin semiconductor," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    3. Hangyong Shan & Ivan Iorsh & Bo Han & Christoph Rupprecht & Heiko Knopf & Falk Eilenberger & Martin Esmann & Kentaro Yumigeta & Kenji Watanabe & Takashi Taniguchi & Sebastian Klembt & Sven Höfling & S, 2022. "Brightening of a dark monolayer semiconductor via strong light-matter coupling in a cavity," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    4. Hangyong Shan & Lukas Lackner & Bo Han & Evgeny Sedov & Christoph Rupprecht & Heiko Knopf & Falk Eilenberger & Johannes Beierlein & Nils Kunte & Martin Esmann & Kentaro Yumigeta & Kenji Watanabe & Tak, 2021. "Spatial coherence of room-temperature monolayer WSe2 exciton-polaritons in a trap," Nature Communications, Nature, vol. 12(1), pages 1-7, December.
    5. Zehua Hu & Tanjung Krisnanda & Antonio Fieramosca & Jiaxin Zhao & Qianlu Sun & Yuzhong Chen & Haiyun Liu & Yuan Luo & Rui Su & Junyong Wang & Kenji Watanabe & Takashi Taniguchi & Goki Eda & Xiao Rensh, 2024. "Energy transfer driven brightening of MoS2 by ultrafast polariton relaxation in microcavity MoS2/hBN/WS2 heterostructures," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    6. Ilia Sokolovskii & Ruth H. Tichauer & Dmitry Morozov & Johannes Feist & Gerrit Groenhof, 2023. "Multi-scale molecular dynamics simulations of enhanced energy transfer in organic molecules under strong coupling," Nature Communications, Nature, vol. 14(1), pages 1-11, December.

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