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Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride

Author

Listed:
  • Clarisse Fournier

    (Université Paris-Saclay, UVSQ, CNRS, GEMaC)

  • Alexandre Plaud

    (Université Paris-Saclay, UVSQ, CNRS, GEMaC)

  • Sébastien Roux

    (Université Paris-Saclay, UVSQ, CNRS, GEMaC)

  • Aurélie Pierret

    (Université PSL, CNRS, Sorbonne Université, Université de Paris)

  • Michael Rosticher

    (Université PSL, CNRS, Sorbonne Université, Université de Paris)

  • Kenji Watanabe

    (National Institute for Materials Science)

  • Takashi Taniguchi

    (National Institute for Materials Science)

  • Stéphanie Buil

    (Université Paris-Saclay, UVSQ, CNRS, GEMaC)

  • Xavier Quélin

    (Université Paris-Saclay, UVSQ, CNRS, GEMaC)

  • Julien Barjon

    (Université Paris-Saclay, UVSQ, CNRS, GEMaC)

  • Jean-Pierre Hermier

    (Université Paris-Saclay, UVSQ, CNRS, GEMaC)

  • Aymeric Delteil

    (Université Paris-Saclay, UVSQ, CNRS, GEMaC)

Abstract

Single photon emitters (SPEs) in low-dimensional layered materials have recently gained a large interest owing to the auspicious perspectives of integration and extreme miniaturization offered by this class of materials. However, accurate control of both the spatial location and the emission wavelength of the quantum emitters is essentially lacking to date, thus hindering further technological steps towards scalable quantum photonic devices. Here, we evidence SPEs in high purity synthetic hexagonal boron nitride (hBN) that can be activated by an electron beam at chosen locations. SPE ensembles are generated with a spatial accuracy better than the cubed emission wavelength, thus opening the way to integration in optical microstructures. Stable and bright single photon emission is subsequently observed in the visible range up to room temperature upon non-resonant laser excitation. Moreover, the low-temperature emission wavelength is reproducible, with an ensemble distribution of width 3 meV, a statistical dispersion that is more than one order of magnitude lower than the narrowest wavelength spreads obtained in epitaxial hBN samples. Our findings constitute an essential step towards the realization of top-down integrated devices based on identical quantum emitters in 2D materials.

Suggested Citation

  • Clarisse Fournier & Alexandre Plaud & Sébastien Roux & Aurélie Pierret & Michael Rosticher & Kenji Watanabe & Takashi Taniguchi & Stéphanie Buil & Xavier Quélin & Julien Barjon & Jean-Pierre Hermier &, 2021. "Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride," Nature Communications, Nature, vol. 12(1), pages 1-6, December.
  • Handle: RePEc:nat:natcom:v:12:y:2021:i:1:d:10.1038_s41467-021-24019-6
    DOI: 10.1038/s41467-021-24019-6
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    Cited by:

    1. T. Thu Ha Do & Milad Nonahal & Chi Li & Vytautas Valuckas & Hark Hoe Tan & Arseniy I. Kuznetsov & Hai Son Nguyen & Igor Aharonovich & Son Tung Ha, 2024. "Room-temperature strong coupling in a single-photon emitter-metasurface system," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    2. Robert Smit & Arash Tebyani & Jil Hameury & Sense Jan van der Molen & Michel Orrit, 2023. "Sharp zero-phonon lines of single organic molecules on a hexagonal boron-nitride surface," Nature Communications, Nature, vol. 14(1), pages 1-8, December.

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