IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v12y2021i1d10.1038_s41467-021-21698-z.html
   My bibliography  Save this article

Inhomogeneous Kondo-lattice in geometrically frustrated Pr2Ir2O7

Author

Listed:
  • Mariam Kavai

    (Binghamton University)

  • Joel Friedman

    (Binghamton University)

  • Kyle Sherman

    (Binghamton University)

  • Mingda Gong

    (Binghamton University)

  • Ioannis Giannakis

    (Binghamton University)

  • Samad Hajinazar

    (Binghamton University)

  • Haoyu Hu

    (Rice University)

  • Sarah E. Grefe

    (Rice University)

  • Justin Leshen

    (Binghamton University)

  • Qiu Yang

    (University of Tokyo)

  • Satoru Nakatsuji

    (University of Tokyo
    University of Tokyo
    University of Tokyo)

  • Aleksey N. Kolmogorov

    (Binghamton University)

  • Qimiao Si

    (Rice University)

  • Michael Lawler

    (Binghamton University)

  • Pegor Aynajian

    (Binghamton University)

Abstract

Magnetic fluctuations induced by geometric frustration of local Ir-spins disturb the formation of long-range magnetic order in the family of pyrochlore iridates. As a consequence, Pr2Ir2O7 lies at a tuning-free antiferromagnetic-to-paramagnetic quantum critical point and exhibits an array of complex phenomena including the Kondo effect, biquadratic band structure, and metallic spin liquid. Using spectroscopic imaging with the scanning tunneling microscope, complemented with machine learning, density functional theory and theoretical modeling, we probe the local electronic states in Pr2Ir2O7 and find an electronic phase separation. Nanoscale regions with a well-defined Kondo resonance are interweaved with a non-magnetic metallic phase with Kondo-destruction. These spatial nanoscale patterns display a fractal geometry with power-law behavior extended over two decades, consistent with being in proximity to a critical point. Our discovery reveals a nanoscale tuning route, viz. using a spatial variation of the electronic potential as a means of adjusting the balance between Kondo entanglement and geometric frustration.

Suggested Citation

  • Mariam Kavai & Joel Friedman & Kyle Sherman & Mingda Gong & Ioannis Giannakis & Samad Hajinazar & Haoyu Hu & Sarah E. Grefe & Justin Leshen & Qiu Yang & Satoru Nakatsuji & Aleksey N. Kolmogorov & Qimi, 2021. "Inhomogeneous Kondo-lattice in geometrically frustrated Pr2Ir2O7," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:12:y:2021:i:1:d:10.1038_s41467-021-21698-z
    DOI: 10.1038/s41467-021-21698-z
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-021-21698-z
    File Function: Abstract
    Download Restriction: no

    File URL: https://libkey.io/10.1038/s41467-021-21698-z?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:12:y:2021:i:1:d:10.1038_s41467-021-21698-z. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    We have no bibliographic references for this item. You can help adding them by using this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.