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Giant voltage-induced modification of magnetism in micron-scale ferromagnetic metals by hydrogen charging

Author

Listed:
  • Xinglong Ye

    (Karlsruhe Institute of Technology)

  • Harish K. Singh

    (Technische Universität Darmstadt)

  • Hongbin Zhang

    (Technische Universität Darmstadt)

  • Holger Geßwein

    (Karlsruhe Institute of Technology)

  • Mohammed Reda Chellali

    (Karlsruhe Institute of Technology)

  • Ralf Witte

    (Karlsruhe Institute of Technology)

  • Alan Molinari

    (Karlsruhe Institute of Technology
    IBM Research – Zurich)

  • Konstantin Skokov

    (Technische Universität Darmstadt)

  • Oliver Gutfleisch

    (Technische Universität Darmstadt)

  • Horst Hahn

    (Karlsruhe Institute of Technology)

  • Robert Kruk

    (Karlsruhe Institute of Technology)

Abstract

Owing to electric-field screening, the modification of magnetic properties in ferromagnetic metals by applying small voltages is restricted to a few atomic layers at the surface of metals. Bulk metallic systems usually do not exhibit any magneto-electric effect. Here, we report that the magnetic properties of micron-scale ferromagnetic metals can be modulated substantially through electrochemically-controlled insertion and extraction of hydrogen atoms in metal structure. By applying voltages of only ~ 1 V, we show that the coercivity of micrometer-sized SmCo5, as a bulk model material, can be reversibly adjusted by ~ 1 T, two orders of magnitudes larger than previously reported. Moreover, voltage-assisted magnetization reversal is demonstrated at room temperature. Our study opens up a way to control the magnetic properties in ferromagnetic metals beyond the electric-field screening length, paving its way towards practical use in magneto-electric actuation and voltage-assisted magnetic storage.

Suggested Citation

  • Xinglong Ye & Harish K. Singh & Hongbin Zhang & Holger Geßwein & Mohammed Reda Chellali & Ralf Witte & Alan Molinari & Konstantin Skokov & Oliver Gutfleisch & Horst Hahn & Robert Kruk, 2020. "Giant voltage-induced modification of magnetism in micron-scale ferromagnetic metals by hydrogen charging," Nature Communications, Nature, vol. 11(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:11:y:2020:i:1:d:10.1038_s41467-020-18552-z
    DOI: 10.1038/s41467-020-18552-z
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