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Extraction of higher-order nonlinear electronic response in solids using high harmonic generation

Author

Listed:
  • Seunghwoi Han

    (Korea Advanced Institute of Science and Technology (KAIST)
    University of Central Florida)

  • Lisa Ortmann

    (Max Planck Institute for the Physics of Complex Systems)

  • Hyunwoong Kim

    (Korea Advanced Institute of Science and Technology (KAIST))

  • Yong Woo Kim

    (Korea Advanced Institute of Science and Technology (KAIST))

  • Takashi Oka

    (Max Planck Institute for the Physics of Complex Systems
    Max Planck Institute for Chemical Physics of Solids)

  • Alexis Chacon

    (Physics and Chemistry of Materials T1-Division, Los Alamos National Laboratory)

  • Brent Doran

    (University of Oxford)

  • Marcelo Ciappina

    (Institute of Physics of the ASCR, ELI-Beamlines)

  • Maciej Lewenstein

    (ICFO – Institut de Ciències Fotòniques, The Barcelona Institute of Science and Technology
    ICREA – Institució Catalana de Recerca i Estudis Avançats)

  • Seung-Woo Kim

    (Korea Advanced Institute of Science and Technology (KAIST))

  • Seungchul Kim

    (Pusan National University)

  • Alexandra S. Landsman

    (Max Planck Institute for the Physics of Complex Systems)

Abstract

Nonlinear susceptibilities are key to ultrafast lightwave driven optoelectronics, allowing petahertz scaling manipulation of the signal. Recent experiments retrieved a 3rd order nonlinear susceptibility by comparing the nonlinear response induced by a strong laser field to a linear response induced by the otherwise identical weak field. The highly nonlinear nature of high harmonic generation (HHG) has the potential to extract even higher order nonlinear susceptibility terms. However, up till now, such characterization has been elusive due to a lack of direct correspondence between high harmonics and nonlinear susceptibilities. Here, we demonstrate a regime where such correspondence can be clearly made, extracting nonlinear susceptibilities (7th, 9th, and 11th) from sapphire of the same order as the measured high harmonics. The extracted high order susceptibilities show angular-resolved periodicities arising from variation in the band structure with crystal orientation. Our results open a door to multi-channel signal processing, controlled by laser polarization.

Suggested Citation

  • Seunghwoi Han & Lisa Ortmann & Hyunwoong Kim & Yong Woo Kim & Takashi Oka & Alexis Chacon & Brent Doran & Marcelo Ciappina & Maciej Lewenstein & Seung-Woo Kim & Seungchul Kim & Alexandra S. Landsman, 2019. "Extraction of higher-order nonlinear electronic response in solids using high harmonic generation," Nature Communications, Nature, vol. 10(1), pages 1-6, December.
    • Handle: RePEc:nat:natcom:v:10:y:2019:i:1:d:10.1038_s41467-019-11096-x
    DOI: 10.1038/s41467-019-11096-x
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    Cited by:

    1. Sylvianne D. C. Roscam Abbing & Nataliia Kuzkova & Roy Linden & Filippo Campi & Brian Keijzer & Corentin Morice & Zhuang-Yan Zhang & Maarten L. S. Geest & Peter M. Kraus, 2024. "Enhancing the efficiency of high-order harmonics with two-color non-collinear wave mixing in silica," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    2. Yang-Yang Lv & Jinlong Xu & Shuang Han & Chi Zhang & Yadong Han & Jian Zhou & Shu-Hua Yao & Xiao-Ping Liu & Ming-Hui Lu & Hongming Weng & Zhenda Xie & Y. B. Chen & Jianbo Hu & Yan-Feng Chen & Shining , 2021. "High-harmonic generation in Weyl semimetal β-WP2 crystals," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    3. Sha Li & Yaguo Tang & Lisa Ortmann & Bradford K. Talbert & Cosmin I. Blaga & Yu Hang Lai & Zhou Wang & Yang Cheng & Fengyuan Yang & Alexandra S. Landsman & Pierre Agostini & Louis F. DiMauro, 2023. "High-order harmonic generation from a thin film crystal perturbed by a quasi-static terahertz field," Nature Communications, Nature, vol. 14(1), pages 1-9, December.

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