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High sensitivity variable-temperature infrared nanoscopy of conducting oxide interfaces

Author

Listed:
  • Weiwei Luo

    (University of Geneva)

  • Margherita Boselli

    (University of Geneva)

  • Jean-Marie Poumirol

    (University of Geneva)

  • Ivan Ardizzone

    (University of Geneva)

  • Jérémie Teyssier

    (University of Geneva)

  • Dirk Marel

    (University of Geneva)

  • Stefano Gariglio

    (University of Geneva)

  • Jean-Marc Triscone

    (University of Geneva)

  • Alexey B. Kuzmenko

    (University of Geneva)

Abstract

Probing the local transport properties of two-dimensional electron systems (2DES) confined at buried interfaces requires a non-invasive technique with a high spatial resolution operating in a broad temperature range. In this paper, we investigate the scattering-type scanning near field optical microscopy as a tool for studying the conducting LaAlO3/SrTiO3 interface from room temperature down to 6 K. We show that the near-field optical signal, in particular its phase component, is highly sensitive to the transport properties of the electron system present at the interface. Our modeling reveals that such sensitivity originates from the interaction of the AFM tip with coupled plasmon–phonon modes with a small penetration depth. The model allows us to quantitatively correlate changes in the optical signal with the variation of the 2DES transport properties induced by cooling and by electrostatic gating. To probe the spatial resolution of the technique, we image conducting nano-channels written in insulating heterostructures with a voltage-biased tip of an atomic force microscope.

Suggested Citation

  • Weiwei Luo & Margherita Boselli & Jean-Marie Poumirol & Ivan Ardizzone & Jérémie Teyssier & Dirk Marel & Stefano Gariglio & Jean-Marc Triscone & Alexey B. Kuzmenko, 2019. "High sensitivity variable-temperature infrared nanoscopy of conducting oxide interfaces," Nature Communications, Nature, vol. 10(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:10:y:2019:i:1:d:10.1038_s41467-019-10672-5
    DOI: 10.1038/s41467-019-10672-5
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    Cited by:

    1. Yixi Zhou & Adrien Waelchli & Margherita Boselli & Iris Crassee & Adrien Bercher & Weiwei Luo & Jiahua Duan & J.L.M. Mechelen & Dirk Marel & Jérémie Teyssier & Carl Willem Rischau & Lukas Korosec & St, 2023. "Thermal and electrostatic tuning of surface phonon-polaritons in LaAlO3/SrTiO3 heterostructures," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    2. Ruijuan Xu & Iris Crassee & Hans A. Bechtel & Yixi Zhou & Adrien Bercher & Lukas Korosec & Carl Willem Rischau & Jérémie Teyssier & Kevin J. Crust & Yonghun Lee & Stephanie N. Gilbert Corder & Jiarui , 2024. "Highly confined epsilon-near-zero and surface phonon polaritons in SrTiO3 membranes," Nature Communications, Nature, vol. 15(1), pages 1-9, December.

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