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Dimensional crossover in a layered ferromagnet detected by spin correlation driven distortions

Author

Listed:
  • A. Ron

    (California Institute of Technology
    California Institute of Technology)

  • E. Zoghlin

    (University of California)

  • L. Balents

    (University of California)

  • S. D. Wilson

    (University of California)

  • D. Hsieh

    (California Institute of Technology
    California Institute of Technology)

Abstract

Magneto-elastic distortions are commonly detected across magnetic long-range ordering (LRO) transitions. In principle, they are also induced by the magnetic short-range ordering (SRO) that precedes a LRO transition, which contains information about short-range correlations and energetics that are essential for understanding how LRO is established. However these distortions are difficult to resolve because the associated atomic displacements are exceedingly small and do not break symmetry. Here we demonstrate high-multipole nonlinear optical polarimetry as a sensitive and mode selective probe of SRO induced distortions using CrSiTe3 as a testbed. This compound is composed of weakly bonded sheets of nearly isotropic ferromagnetically interacting spins that, in the Heisenberg limit, would individually be impeded from LRO by the Mermin-Wagner theorem. Our results show that CrSiTe3 evades this law via a two-step crossover from two- to three-dimensional magnetic SRO, manifested through two successive and previously undetected totally symmetric distortions above its Curie temperature.

Suggested Citation

  • A. Ron & E. Zoghlin & L. Balents & S. D. Wilson & D. Hsieh, 2019. "Dimensional crossover in a layered ferromagnet detected by spin correlation driven distortions," Nature Communications, Nature, vol. 10(1), pages 1-6, December.
  • Handle: RePEc:nat:natcom:v:10:y:2019:i:1:d:10.1038_s41467-019-09663-3
    DOI: 10.1038/s41467-019-09663-3
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    Cited by:

    1. Matan Even Tzur & Ofer Neufeld & Eliyahu Bordo & Avner Fleischer & Oren Cohen, 2022. "Selection rules in symmetry-broken systems by symmetries in synthetic dimensions," Nature Communications, Nature, vol. 13(1), pages 1-10, December.

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