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Liquid metal-filled magnetorheological elastomer with positive piezoconductivity

Author

Listed:
  • Guolin Yun

    (University of Wollongong)

  • Shi-Yang Tang

    (University of Wollongong)

  • Shuaishuai Sun

    (University of Wollongong)

  • Dan Yuan

    (University of Wollongong)

  • Qianbin Zhao

    (University of Wollongong)

  • Lei Deng

    (University of Wollongong)

  • Sheng Yan

    (The University of Tokyo)

  • Haiping Du

    (University of Wollongong)

  • Michael D. Dickey

    (North Carolina State University)

  • Weihua Li

    (University of Wollongong)

Abstract

Conductive elastic composites have been used widely in soft electronics and soft robotics. These composites are typically a mixture of conductive fillers within elastomeric substrates. They can sense strain via changes in resistance resulting from separation of the fillers during elongation. Thus, most elastic composites exhibit a negative piezoconductive effect, i.e. the conductivity decreases under tensile strain. This property is undesirable for stretchable conductors since such composites may become less conductive during deformation. Here, we report a liquid metal-filled magnetorheological elastomer comprising a hybrid of fillers of liquid metal microdroplets and metallic magnetic microparticles. The composite’s resistivity reaches a maximum value in the relaxed state and drops drastically under any deformation, indicating that the composite exhibits an unconventional positive piezoconductive effect. We further investigate the magnetic field-responsive thermal properties of the composite and demonstrate several proof-of-concept applications. This composite has prospective applications in sensors, stretchable conductors, and responsive thermal interfaces.

Suggested Citation

  • Guolin Yun & Shi-Yang Tang & Shuaishuai Sun & Dan Yuan & Qianbin Zhao & Lei Deng & Sheng Yan & Haiping Du & Michael D. Dickey & Weihua Li, 2019. "Liquid metal-filled magnetorheological elastomer with positive piezoconductivity," Nature Communications, Nature, vol. 10(1), pages 1-9, December.
  • Handle: RePEc:nat:natcom:v:10:y:2019:i:1:d:10.1038_s41467-019-09325-4
    DOI: 10.1038/s41467-019-09325-4
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    Cited by:

    1. Gun-Hee Lee & Ye Rim Lee & Hanul Kim & Do A Kwon & Hyeonji Kim & Congqi Yang & Siyoung Q. Choi & Seongjun Park & Jae-Woong Jeong & Steve Park, 2022. "Rapid meniscus-guided printing of stable semi-solid-state liquid metal microgranular-particle for soft electronics," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    2. Haojie Jiang & Bin Yuan & Hongtao Guo & Fei Pan & Fanmao Meng & Yongpeng Wu & Xiao Wang & Lingyang Ruan & Shuhuai Zheng & Yang Yang & Zheng Xiu & Lixin Li & Changsheng Wu & Yongqing Gong & Menghao Yan, 2024. "Malleable, printable, bondable, and highly conductive MXene/liquid metal plasticine with improved wettability," Nature Communications, Nature, vol. 15(1), pages 1-12, December.

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