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Optimization of Solidification and Stabilization Efficiency of Heavy Metal Contaminated Sediment Based on Response Surface Methodology

Author

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  • Yang Yang

    (School of Environment and Architecture, University of Shanghai for Science and Technology, Shanghai 200093, China)

  • Moting Li

    (School of Environment and Architecture, University of Shanghai for Science and Technology, Shanghai 200093, China)

  • Yan Sun

    (School of Environment and Architecture, University of Shanghai for Science and Technology, Shanghai 200093, China)

  • Huimin Gao

    (School of Environment and Architecture, University of Shanghai for Science and Technology, Shanghai 200093, China)

  • Lingchen Mao

    (School of Environment and Architecture, University of Shanghai for Science and Technology, Shanghai 200093, China)

  • He Zhang

    (School of Environment and Architecture, University of Shanghai for Science and Technology, Shanghai 200093, China)

  • Hong Tao

    (School of Environment and Architecture, University of Shanghai for Science and Technology, Shanghai 200093, China)

Abstract

Solidification and stabilization (S/S) by agents and stabilizers is an effective way to treat heavy metal-contaminated sediments. Optimization of curing condition is crucial to minimize the consumption of reagents on the base of effective S/S. In this work, the synergistic effects of cement and stabilizer on mechanical strength and leaching toxicity of contaminated sediments were investigated, and the S/S conditions were optimized using response surface methodology. On the basis of a single-factor test, multi-factor experiments were conducted to fit the relationship between the S/S effect of contaminated sediments and the amount of cement and stabilizer. The mechanism of stabilization was investigated by the results from the revised BCR method. The results indicate that the optimal curing conditions were 44.29% of cement content with 2.05% of trimercapto-s-triazine trisodium salt (TMT). After 28 days of curing, the compressive strength reached 2.07 MPa and the leaching concentrations of Cd, Cu, and Pb were 0.094 mg/L, 0.031 mg/L, and 0.173 mg/L, respectively, which met the requirement of in-situ resource recycling standard. The stability of heavy metals was significantly improved as a result of the removal of acid extractable fraction (15.58~69.92%) and an increase in the residual fraction (18.27~49.07%).

Suggested Citation

  • Yang Yang & Moting Li & Yan Sun & Huimin Gao & Lingchen Mao & He Zhang & Hong Tao, 2022. "Optimization of Solidification and Stabilization Efficiency of Heavy Metal Contaminated Sediment Based on Response Surface Methodology," Sustainability, MDPI, vol. 14(6), pages 1-10, March.
  • Handle: RePEc:gam:jsusta:v:14:y:2022:i:6:p:3306-:d:769206
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    References listed on IDEAS

    as
    1. Mert Guney & Zhanel Akimzhanova & Aiganym Kumisbek & Symbat Kismelyeva & Almira Guney & Ferhat Karaca & Vassilis Inglezakis, 2021. "Assessment of Distribution of Potentially Toxic Elements in Different Environmental Media Impacted by a Former Chlor-Alkali Plant," Sustainability, MDPI, vol. 13(24), pages 1-26, December.
    2. Vemula Anand Reddy & Chandresh H. Solanki & Shailendra Kumar & Krishna R. Reddy & Yan-Jun Du, 2020. "Stabilization/Solidification of Zinc- and Lead-Contaminated Soil Using Limestone Calcined Clay Cement (LC 3 ): An Environmentally Friendly Alternative," Sustainability, MDPI, vol. 12(9), pages 1-13, May.
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    Cited by:

    1. Zhitong Yao & Wei Qi & José Luiz Francisco Alves, 2023. "Editorial for the Special Issue on the Environmentally Friendly Management and Treatment of Solid Waste to Approach Zero Waste City," Sustainability, MDPI, vol. 15(1), pages 1-2, January.

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