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Observation of Dispersion in the Japanese Coastal Area of Released 90 Sr, 134 Cs, and 137 Cs from the Fukushima Daiichi Nuclear Power Plant to the Sea in 2013

Author

Listed:
  • Hirofumi Tazoe

    (Department of Radiation Chemistry, Institute of Radiation Emergency Mediation, Hirosaki University, Hirosaki 036-8652, Japan)

  • Takeyasu Yamagata

    (College of Humanities and Sciences, Nihon University, Tokyo 156-8550, Japan)

  • Kazuki Tsujita

    (Graduate School of Basic Integrated Sciences, Nihon University, Tokyo 156-8550, Japan)

  • Hisao Nagai

    (College of Humanities and Sciences, Nihon University, Tokyo 156-8550, Japan)

  • Hajime Obata

    (Atmosphere and Ocean Research Institute, University of Tokyo 277-8564, Japan)

  • Daisuke Tsumune

    (Environmental Science Research Laboratory, Central Research Institute of Electric Power Industry, Tokyo 270-1194, Japan)

  • Jota Kanda

    (Department of Ocean Sciences, Graduate Faculty of Marine Science, Tokyo University of Marine Science and Technology, Tokyo 108-8477, Japan)

  • Masatoshi Yamada

    (Department of Radiation Chemistry, Institute of Radiation Emergency Mediation, Hirosaki University, Hirosaki 036-8652, Japan
    Marine Ecology Research Institute, Chiba 299-5105, Japan)

Abstract

The March 2011 earthquake and tsunami resulted in significant damage to the Fukushima Daiichi Nuclear Power Plant (FDNPP) and the subsequent release of radionuclides into the ocean. Here, we investigated the spatial distribution of strontium-90 ( 90 Sr) and cesium-134/cesium-137 ( 134, 137 Cs) in surface seawater of the coastal region near the FDNPP. In the coastal region, 90 Sr activity was high, from 0.89 to 29.13 mBq L −1 , with detectable FDNPP site-derived 134 Cs. This indicated that release of 90 Sr from the power plant was ongoing even in May 2013, as was that of 134 Cs and 137 Cs. 90 Sr activities measured at open ocean sites corresponded to background derived from atmospheric nuclear weapons testing fallout. The FDNPP site-derived 90 Sr/ 137 Cs activity ratios in seawater were much higher than those in the direct discharge event in March 2011, in river input, and in seabed sediment; those ratios showed large variability, ranging from 0.16 to 0.64 despite a short sampling period. This FDNPP site-derived 90 Sr/ 137 Cs activity ratio suggests that these radionuclides were mainly derived from stagnant water in the reactor and turbine buildings of the FDNPP, while a different source with a low 90 Sr/ 137 Cs ratio could contribute to and produce the temporal variability of the 90 Sr/ 137 Cs ratio in coastal water. We estimated the release rate of 90 Sr from the power plant as 9.6 ± 6.1 GBq day −1 in May 2013 on the basis of the relationship between 90 Sr and 137 Cs activity ( 90 Sr/ 137 Cs = 0.66 ± 0.05) and 137 Cs release rate.

Suggested Citation

  • Hirofumi Tazoe & Takeyasu Yamagata & Kazuki Tsujita & Hisao Nagai & Hajime Obata & Daisuke Tsumune & Jota Kanda & Masatoshi Yamada, 2019. "Observation of Dispersion in the Japanese Coastal Area of Released 90 Sr, 134 Cs, and 137 Cs from the Fukushima Daiichi Nuclear Power Plant to the Sea in 2013," IJERPH, MDPI, vol. 16(21), pages 1-15, October.
    • Handle: RePEc:gam:jijerp:v:16:y:2019:i:21:p:4094-:d:279741
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    Citations

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    Cited by:

    1. Taisir Khudhair Abbas & Thaeerh Tariq Abdulghafoor & Ali Hassan Aziz & Saad Al-Saadi & Takrid Munam Nafae & Khalid Turki Rashid & Qusay F. Alsalhy, 2023. "Investigation of the Segregation of Radiocesium from Contaminated Aqueous Waste Using AMP-PAN Extraction Chromatography," Energies, MDPI, vol. 16(18), pages 1-13, September.
    2. Yiyao Cao & Lei Zhou & Hong Ren & Hua Zou, 2022. "Determination, Separation and Application of 137 Cs: A Review," IJERPH, MDPI, vol. 19(16), pages 1-15, August.

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