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An experimental investigation of coupled chemico-mineralogical and mechanical changes in varyingly-cemented sandstones upon CO2 injection in deep saline aquifer environments

Author

Listed:
  • Rathnaweera, T.D.
  • Ranjith, P.G.
  • Perera, M.S.A.
  • Ranathunga, A.S.
  • Wanniarachchi, W.A.M.
  • Yang, S.Q.
  • Lashin, A.
  • Al Arifi, N.

Abstract

Although CO2 storage in deep saline aquifers is now accepted as a potential option for atmospheric CO2 mitigation, the chemico-mineralogical property alterations in the aquifer formation associated with CO2/brine/rock mineral interactions, the corresponding influence on formation hydro-mechanical properties and the effect of rock mineral structure, are not yet fully understood. This study was therefore conducted to obtain a comprehensive understanding of the effect of long-term CO2 exposure on the chemico-mineralogical structure and corresponding strength characteristics of saline aquifer rock formations using silicate cement (SS) and carbonate cement (CS) Hawkesbury sandstone samples collected from the Sydney basin. Sandstone samples were first reacted with brine+CO2 under different injection pressures (both sub-critical (4, 6 MPa) and super-critical (8, 10 MPa)) under a constant temperature of 35 °C. A comprehensive chemico-mineralogical analysis (ICP-AES and XRD) was first conducted on both the rock mass pore fluid and the rock matrix over the saturation period of one year, giving special attention to the alteration of dominant rock minerals (quartz, calcite and kaolinite). The overall influence after 12 months of saturation with brine and CO2 on the strength characteristics of the two types of sandstones (SS and CS) was then investigated and correlated with the chemico-mineralogical reaction, in order to understand the coupled process.

Suggested Citation

  • Rathnaweera, T.D. & Ranjith, P.G. & Perera, M.S.A. & Ranathunga, A.S. & Wanniarachchi, W.A.M. & Yang, S.Q. & Lashin, A. & Al Arifi, N., 2017. "An experimental investigation of coupled chemico-mineralogical and mechanical changes in varyingly-cemented sandstones upon CO2 injection in deep saline aquifer environments," Energy, Elsevier, vol. 133(C), pages 404-414.
    • Handle: RePEc:eee:energy:v:133:y:2017:i:c:p:404-414
    DOI: 10.1016/j.energy.2017.05.154
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    Cited by:

    1. Vafaie, Atefeh & Cama, Jordi & Soler, Josep M. & Kivi, Iman R. & Vilarrasa, Victor, 2023. "Chemo-hydro-mechanical effects of CO2 injection on reservoir and seal rocks: A review on laboratory experiments," Renewable and Sustainable Energy Reviews, Elsevier, vol. 178(C).
    2. Dabbaghi, Ehsan & Ng, Kam, 2024. "Effects of CO2 on the mineralogy, mechanical, and transport properties of rocks," Renewable and Sustainable Energy Reviews, Elsevier, vol. 199(C).
    3. Du, Shuheng & Shi, Yongmin & Zheng, Xiaojiao & Chai, Guangsheng, 2020. "Using “Umbrella Deconstruction & Energy Dispersive Spectrometer (UD-EDS)” technique to quantify the anisotropic elements distribution of "Chang 7" shale and its significance," Energy, Elsevier, vol. 191(C).
    4. Zhidi Wu & Jason D. Simmons & Samuel Otu & Alex Rinehart & Andrew Luhmann & Jason Heath & Peter Mozley & Bhaskar S. Majumdar, 2023. "Control of Cement Timing, Mineralogy, and Texture on Hydro-chemo-mechanical Coupling from CO 2 Injection into Sandstone: A Synthesis," Energies, MDPI, vol. 16(24), pages 1-27, December.
    5. Bo Liu & Fangyuan Zhao & Jinpeng Xu & Yueming Qi, 2019. "Experimental Investigation and Numerical Simulation of CO 2 –Brine–Rock Interactions during CO 2 Sequestration in a Deep Saline Aquifer," Sustainability, MDPI, vol. 11(2), pages 1-18, January.

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