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A pilot study of activated carbon and metal–organic frameworks for methane storage

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  • Beckner, Matthew
  • Dailly, Anne

Abstract

The methane storage of an activated carbon and two metal–organic frameworks (Cu3(btc)2 and Al(OH) Fumarate) are compared for laboratory scale (∼1g of material) to pilot scale measurements (∼1.5kg of material). Excess adsorption and volumetric storage capacity uptakes agreed well between the two measurements. By decomposing the volumetric storage capacity into the contributions from the gas and adsorbed phases, the volumetric storage was evidenced to be dominated by the excess adsorption up to 100bar. The volumetric storage is a function of both the excess adsorption uptake and the material’s bulk density. The AC shows higher heat transfer rates than the metal–organic frameworks upon adsorption indicating a superior thermal conductivity. The mean flow velocity has been estimated from the pilot scale measurements and is discussed as it will strongly influence the adsorbed natural gas technology performance.

Suggested Citation

  • Beckner, Matthew & Dailly, Anne, 2016. "A pilot study of activated carbon and metal–organic frameworks for methane storage," Applied Energy, Elsevier, vol. 162(C), pages 506-514.
  • Handle: RePEc:eee:appene:v:162:y:2016:i:c:p:506-514
    DOI: 10.1016/j.apenergy.2015.10.110
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    References listed on IDEAS

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    1. Beckner, Matthew & Dailly, Anne, 2015. "Adsorbed methane storage for vehicular applications," Applied Energy, Elsevier, vol. 149(C), pages 69-74.
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    Cited by:

    1. Mitra, Sourav & Thu, Kyaw & Saha, Bidyut Baran & Dutta, Pradip, 2017. "Performance evaluation and determination of minimum desorption temperature of a two-stage air cooled silica gel/water adsorption system," Applied Energy, Elsevier, vol. 206(C), pages 507-518.
    2. Papakokkinos, Giorgos & Castro, Jesús & López, Joan & Oliva, Assensi, 2019. "A generalized computational model for the simulation of adsorption packed bed reactors – Parametric study of five reactor geometries for cooling applications," Applied Energy, Elsevier, vol. 235(C), pages 409-427.
    3. Byamba-Ochir, Narandalai & Shim, Wang Geun & Balathanigaimani, M.S. & Moon, Hee, 2017. "High density Mongolian anthracite based porous carbon monoliths for methane storage by adsorption," Applied Energy, Elsevier, vol. 190(C), pages 257-265.
    4. Nima Mohammadi & Behnam Mousazadeh & Touba Hamoule, 2021. "Synthesis and characterization of NH2-SiO2@Cu-MOF as a high-performance adsorbent for Pb ion removal from water environment," Environment, Development and Sustainability: A Multidisciplinary Approach to the Theory and Practice of Sustainable Development, Springer, vol. 23(2), pages 1688-1705, February.
    5. Tong, Wen & Lv, Yongqin & Svec, Frantisek, 2016. "Advantage of nanoporous styrene-based monolithic structure over beads when applied for methane storage," Applied Energy, Elsevier, vol. 183(C), pages 1520-1527.

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